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• W4285402985 endingPage "121715" @default.
• W4285402985 startingPage "121715" @default.
• W4285402985 abstract "• A 3D flower like Ti 3 C 2 /Bi 2 WO 6 with 2D/2D heterojunction was constructed. • The 2D/2D heterojunction contributed to the enhanced interaction at interface. • The physical and photoelectrochemical properties were improved a lot. • h + , O 2 − and OH were active species and the h + was predominant. Constructing 2D/2D heterojunction in traditional metal oxide photocatalyst is considered to be a practical strategy for boosting visible light-driven photocatalytic activity remarkably. This work fabricated 2D/2D heterojunction by decorating 2D Ti 3 C 2 on nanosheet units in 3D flower-like Bi 2 WO 6 hierarchical structure and significantly improved efficiency of photocatalysis degradation of tetracycline hydrochloride (TC-HCl) as a model antibiotic. It is possible to contribute to the constructed interfacial connection between [Bi 2 O 2 ] 2+ layer and Ti 3 C 2 as well as the resulting electron dislocation of Bi-O bonds, which extended light harvesting range, improved photo-generated holes oxidation and accelerated charge transfer. The best rate constant degradation of TC-HCl and TOC removal efficiency were achieved on 3 %-Ti 3 C 2 /Bi 2 WO 6 sample, which were 7 times and 3.5 times that of original Bi 2 WO 6 sample. To gain more insight details about photocatalytic process, reactive species were also investigated and a logical mechanism of TC-HCl degradation was presented. This work demonstrated an intriguing exploration strategy of photo-degradation catalyst and was expected to promote the environmental application of solar-driven antibiotics degradation technology." @default.
• W4285402985 created "2022-07-14" @default.
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• W4285402985 date "2022-10-01" @default.
• W4285402985 modified "2023-10-18" @default.
• W4285402985 title "Decorating 2D Ti3C2 on flower-like hierarchical Bi2WO6 for the 2D/2D heterojunction construction towards photodegradation of tetracycline antibiotics" @default.
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• W4285402985 doi "https://doi.org/10.1016/j.seppur.2022.121715" @default.
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