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- W4285490861 abstract "${mathrm{VO}}_{2}$, of interest for decades due to both its phenomenology and its potential applications, has a monoclinic distortion of the rutile crystal structure at ambient temperature that is coupled to its metal-insulator transition. In contrast, ${mathrm{RuO}}_{2}$ has three electrons more per formula unit, is a metallic conductor, and has an undistorted rutile structure. Here, we report a systematic study of Ru-doped ${mathrm{VO}}_{2}$ (${mathrm{V}}_{1text{ensuremath{-}}x}{mathrm{Ru}}_{x}{mathrm{O}}_{2}, 0.01ensuremath{le}xensuremath{le}0.9)$, generally characterizing its crystal structure, magnetic and electronic properties, and heat capacity. The composition-dependent Wilson ratio is determined. We find that an unusually high Ru doping value (80%, $x=0.8$) is required to achieve a metallic state in ${mathrm{V}}_{1text{ensuremath{-}}x}{mathrm{Ru}}_{x}{mathrm{O}}_{2}$. No superconductivity was observed down to 0.1 K in the metallic materials. We propose a possible understanding for how the insulating state can exist in ${mathrm{V}}_{1text{ensuremath{-}}x}{mathrm{Ru}}_{x}{mathrm{O}}_{2}$ at high Ru contents." @default.
- W4285490861 created "2022-07-15" @default.
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- W4285490861 date "2022-07-15" @default.
- W4285490861 modified "2023-09-24" @default.
- W4285490861 title "Metal-insulator transition and anomalous lattice parameters changes in Ru-doped <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:msub><mml:mi>VO</mml:mi><mml:mn>2</mml:mn></mml:msub></mml:math>" @default.
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- W4285490861 doi "https://doi.org/10.1103/physrevmaterials.6.075005" @default.
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