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• W4285494430 endingPage "8804" @default.
• W4285494430 startingPage "8794" @default.
• W4285494430 abstract "Hierarchical assemblies of functional polymer particles are promising due to their surface as well as physicochemical properties. However, hierarchical composites are complex and challenging to form due to the many steps necessary for integrating different components into one system. Highly structured four-level composite particles were formed in a four-step process. First of all, gold (Au) nanoparticles, poly(methyl methacrylate) (PMMA) nanoparticles, and poly(tripropylene glycol diacrylate) (poly-TPGDA) microparticles were individually synthesized. By applying microfluidic techniques, polymer nano- and microparticles were formed with tunable size and surface properties. Afterwards, the negatively charged gold nanoparticles and PMMA particles functionalized with a positively charged surface were mixed to form Au/PMMA assemblies. The Au/PMMA composites were mixed and incubated with poly-TPGDA microparticles to form ternary Au/PMMA/poly-TPGDA assemblies. For the formation of composite-containing microparticles, Au/PMMA/poly-TPGDA composites were dispersed in an aqueous acrylamide–methylenebisacrylamide solution. Monomer droplets were formed in a co-flow microfluidic device and photopolymerized by UV light. In this way, hierarchically structured four-level composites consisting of four different size ranges─0.025/0.8/30/1000 μm─were obtained. By functionalizing polymer nano- and microparticles with different fluorescent dyes, it was possible to visualize the same composite particle under two different excitation modes (λex = 395–440 and λex = 510–560 nm). The Au/PMMA/poly-TPGDA composite-embedded polyacrylamide microparticles can be potentially used as a model for the creation of composite particles for sensing, catalysis, multilabeling, and biomedical applications." @default.
• W4285494430 created "2022-07-15" @default.
• W4285494430 creator A5026612853 @default.
• W4285494430 creator A5031692081 @default.
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• W4285494430 date "2022-07-14" @default.
• W4285494430 modified "2023-10-02" @default.
• W4285494430 title "Four-Level Structural Hierarchy: Microfluidically Supported Synthesis of Polymer Particle Architectures Incorporating Fluorescence-Labeled Components and Metal Nanoparticles" @default.
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• W4285494430 doi "https://doi.org/10.1021/acs.langmuir.2c00686" @default.
• W4285494430 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/35833738" @default.
• W4285494430 hasPublicationYear "2022" @default.
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