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- W4285521367 startingPage "2021" @default.
- W4285521367 abstract "Although substantial progress has been made for the development of reaction mechanisms for syngas combustion, most previous studies focus on air-fuel conditions. The chemical kinetics under oxy-fuel conditions is significantly different from air-fuel conditions due to the effect of high CO2 concentrations. The present study proposes a new 16-species, 12-step reduced mechanism for syngas combustion and NO-reburning under both air and oxy-fuel conditions by systematical mechanism evaluation, reduction, and validation. Firstly, based on a large set of experimental data of syngas oxy-fuel combustion, including ignition delay times (180 data points in 5 datasets), laminar flame speeds (334 data points in 8 datasets), species concentrations (114 data points from a flow reactor and 558 data points from our jet stirring reactor), 16 existing frequently-used syngas mechanisms are evaluated for both the fuel oxidation and NO reburning. Secondly, the optimal detailed mechanism is thoroughly reduced by both skeletal and time-scale methods. Finally, the reduced mechanism is validated with the detailed mechanism as well as experiments in predictions of ignition, flame propagation, concentration prediction, and extinction. The relative errors between the reduced and detailed mechanisms are less than 10%." @default.
- W4285521367 created "2022-07-16" @default.
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- W4285521367 date "2021-01-01" @default.
- W4285521367 modified "2023-09-26" @default.
- W4285521367 title "Evaluation, development, and validation of a new reduced mechanism for syngas oxidation and NO-reburning under air and oxy-fuel combustion" @default.
- W4285521367 doi "https://doi.org/10.1299/jsmeicope.2021.15.2021-0283" @default.
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