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- W4285604857 abstract "Strong metal-support interactions (SMSIs), one of the core concepts in the field of catalysis, have a substantial influence on catalytic performance, especially stability. Conventional view holds that only reducible metal-oxide supports could induce a SMSI encapsulation state upon high-temperature treatments. Herein, we demonstrate a high-temperature SMSI between platinum and sulfur-doped carbon (S-C) supports, featuring charge transfer, suppression of H2/CO adsorption, and support of encapsulation. We find that the strong chemical interaction between platinum and sulfur atoms greatly suppresses platinum sintering at moderate temperatures of 300°C–700°C, along with the subsequent formation of SMSI encapsulation structures at high temperatures of 900°C–1,100°C. The high-temperature SMSI endowed the Pt/S-C catalysts with outstanding sintering resistance up to 1,100°C and enhanced electrocatalytic oxygen-reduction reaction (ORR) durability in H2–air proton-exchange membrane fuel cells (PEMFCs)." @default.
- W4285604857 created "2022-07-16" @default.
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- W4285604857 date "2022-08-01" @default.
- W4285604857 modified "2023-10-01" @default.
- W4285604857 title "Ultra-high-temperature strong metal-support interactions in carbon-supported catalysts" @default.
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- W4285604857 doi "https://doi.org/10.1016/j.xcrp.2022.100984" @default.
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