Matches in SemOpenAlex for { <https://semopenalex.org/work/W4285729299> ?p ?o ?g. }
- W4285729299 endingPage "13173" @default.
- W4285729299 startingPage "13163" @default.
- W4285729299 abstract "Hydrogen production from water electrolysis in neutral-pH electrolytes can not only avoid the corrosion and safety issues and expand the catalyst option but also potentially integrate with artificial photosynthesis and bioelectrocatalysis. However, heterogeneous catalysts that can efficiently negotiate the sluggish oxygen evolution reaction (OER) in neutral solutions are considerably lacking. Herein, we report a template-assisted strategy for the synthesis of 13 kinds of tube-like nanostructured perovskite oxides (TNPOs) with markedly high Brunauer–Emmett–Teller surface areas. By systematic examination of these TNPOs, we found that the OER activity of TNPOs in neutral solution exhibits a volcano shape as a function of the covalency of transition metal–oxygen bonds. Consequently, our designed Sm-doped LaCoO3 catalyst yields a geometric current density of 8.5 mA cm–2 at 1.75 V versus the reversible hydrogen electrode in 1 M phosphate buffer solution (pH 7) due to the optimized covalency of Co 3d and O 2p states, representing the most active noble-metal-free OER catalyst in neutral electrolytes reported as yet." @default.
- W4285729299 created "2022-07-18" @default.
- W4285729299 creator A5003256124 @default.
- W4285729299 creator A5004147146 @default.
- W4285729299 creator A5005755676 @default.
- W4285729299 creator A5018140110 @default.
- W4285729299 creator A5025431572 @default.
- W4285729299 creator A5027058616 @default.
- W4285729299 creator A5029789751 @default.
- W4285729299 creator A5036055317 @default.
- W4285729299 creator A5036519850 @default.
- W4285729299 creator A5048918848 @default.
- W4285729299 creator A5052676364 @default.
- W4285729299 creator A5074891139 @default.
- W4285729299 creator A5076291539 @default.
- W4285729299 date "2022-07-18" @default.
- W4285729299 modified "2023-10-15" @default.
- W4285729299 title "General Synthesis of Tube-like Nanostructured Perovskite Oxides with Tunable Transition Metal–Oxygen Covalency for Efficient Water Electrooxidation in Neutral Media" @default.
- W4285729299 cites W1757224988 @default.
- W4285729299 cites W1963597613 @default.
- W4285729299 cites W1966029540 @default.
- W4285729299 cites W1967166549 @default.
- W4285729299 cites W1970127494 @default.
- W4285729299 cites W1971800449 @default.
- W4285729299 cites W1972673502 @default.
- W4285729299 cites W1976204697 @default.
- W4285729299 cites W1981368803 @default.
- W4285729299 cites W1986731219 @default.
- W4285729299 cites W1989703096 @default.
- W4285729299 cites W1994887543 @default.
- W4285729299 cites W2020007931 @default.
- W4285729299 cites W2032533160 @default.
- W4285729299 cites W2033507953 @default.
- W4285729299 cites W2075867768 @default.
- W4285729299 cites W2076968595 @default.
- W4285729299 cites W2083222334 @default.
- W4285729299 cites W2100120423 @default.
- W4285729299 cites W2114729935 @default.
- W4285729299 cites W2118976774 @default.
- W4285729299 cites W2120456504 @default.
- W4285729299 cites W2133406747 @default.
- W4285729299 cites W2204347736 @default.
- W4285729299 cites W2224665581 @default.
- W4285729299 cites W2281127889 @default.
- W4285729299 cites W2310142985 @default.
- W4285729299 cites W2317326623 @default.
- W4285729299 cites W2344308937 @default.
- W4285729299 cites W2403509034 @default.
- W4285729299 cites W2510136453 @default.
- W4285729299 cites W2514157351 @default.
- W4285729299 cites W2547752795 @default.
- W4285729299 cites W2592990619 @default.
- W4285729299 cites W2735404343 @default.
- W4285729299 cites W2751722833 @default.
- W4285729299 cites W2767331214 @default.
- W4285729299 cites W2770867421 @default.
- W4285729299 cites W2807996528 @default.
- W4285729299 cites W2810705669 @default.
- W4285729299 cites W2894870637 @default.
- W4285729299 cites W2903072898 @default.
- W4285729299 cites W2936675706 @default.
- W4285729299 cites W2953681281 @default.
- W4285729299 cites W2967299079 @default.
- W4285729299 cites W2970846566 @default.
- W4285729299 cites W2972341275 @default.
- W4285729299 cites W3012236500 @default.
- W4285729299 cites W3022807741 @default.
- W4285729299 cites W3034197579 @default.
- W4285729299 cites W3098733654 @default.
- W4285729299 cites W3175002872 @default.
- W4285729299 cites W4213042605 @default.
- W4285729299 cites W4248958894 @default.
- W4285729299 doi "https://doi.org/10.1021/jacs.2c02989" @default.
- W4285729299 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/35849786" @default.
- W4285729299 hasPublicationYear "2022" @default.
- W4285729299 type Work @default.
- W4285729299 citedByCount "25" @default.
- W4285729299 countsByYear W42857292992022 @default.
- W4285729299 countsByYear W42857292992023 @default.
- W4285729299 crossrefType "journal-article" @default.
- W4285729299 hasAuthorship W4285729299A5003256124 @default.
- W4285729299 hasAuthorship W4285729299A5004147146 @default.
- W4285729299 hasAuthorship W4285729299A5005755676 @default.
- W4285729299 hasAuthorship W4285729299A5018140110 @default.
- W4285729299 hasAuthorship W4285729299A5025431572 @default.
- W4285729299 hasAuthorship W4285729299A5027058616 @default.
- W4285729299 hasAuthorship W4285729299A5029789751 @default.
- W4285729299 hasAuthorship W4285729299A5036055317 @default.
- W4285729299 hasAuthorship W4285729299A5036519850 @default.
- W4285729299 hasAuthorship W4285729299A5048918848 @default.
- W4285729299 hasAuthorship W4285729299A5052676364 @default.
- W4285729299 hasAuthorship W4285729299A5074891139 @default.
- W4285729299 hasAuthorship W4285729299A5076291539 @default.
- W4285729299 hasConcept C106773901 @default.
- W4285729299 hasConcept C127413603 @default.
- W4285729299 hasConcept C135473242 @default.
- W4285729299 hasConcept C147789679 @default.
- W4285729299 hasConcept C155011858 @default.