Matches in SemOpenAlex for { <https://semopenalex.org/work/W4285743376> ?p ?o ?g. }
- W4285743376 abstract "Abstract We investigate the strong-field ion emission from the surface of isolated silica nanoparticles aerosolized from an alcoholic solution, and demonstrate the applicability of the recently reported near-field imaging at 720 nm [Rupp et al., Nat. Comm., 10(1):4655, 2019] to longer wavelength (2 $$mu $$ <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML> <mml:mi>μ</mml:mi> </mml:math> m) and polarizations with arbitrary ellipticity. Based on the experimental observations, we discuss the validity of a previously introduced semi-classical model, which is based on near-field driven charge generation by a Monte-Carlo approach and classical propagation. We furthermore clarify the role of the solvent in the surface composition of the nanoparticles in the interaction region. We find that upon injection of the nanoparticles into the vacuum, the alcoholic solvent evaporates on millisecond time scales, and that the generated ions originate predominantly from covalent bonds with the silica surface rather than from physisorbed solvent molecules. These findings have important implications for the development of future theoretical models of the strong-field ion emission from silica nanoparticles, and the application of near-field imaging and reaction dynamics of functional groups on isolated nanoparticles. Graphical abstract" @default.
- W4285743376 created "2022-07-18" @default.
- W4285743376 creator A5001069974 @default.
- W4285743376 creator A5009223920 @default.
- W4285743376 creator A5014009587 @default.
- W4285743376 creator A5023741536 @default.
- W4285743376 creator A5027797652 @default.
- W4285743376 creator A5042304241 @default.
- W4285743376 creator A5049936709 @default.
- W4285743376 creator A5056949461 @default.
- W4285743376 creator A5057184832 @default.
- W4285743376 creator A5087798025 @default.
- W4285743376 date "2022-06-01" @default.
- W4285743376 modified "2023-09-25" @default.
- W4285743376 title "Imaging elliptically polarized infrared near-fields on nanoparticles by strong-field dissociation of functional surface groups" @default.
- W4285743376 cites W1460138989 @default.
- W4285743376 cites W1974116241 @default.
- W4285743376 cites W1974210390 @default.
- W4285743376 cites W2001610435 @default.
- W4285743376 cites W2045276693 @default.
- W4285743376 cites W2048687775 @default.
- W4285743376 cites W2052679793 @default.
- W4285743376 cites W2073035216 @default.
- W4285743376 cites W2089124524 @default.
- W4285743376 cites W2090651654 @default.
- W4285743376 cites W2094773318 @default.
- W4285743376 cites W2320062826 @default.
- W4285743376 cites W2328557653 @default.
- W4285743376 cites W2341677979 @default.
- W4285743376 cites W2619808832 @default.
- W4285743376 cites W2748174702 @default.
- W4285743376 cites W2808508534 @default.
- W4285743376 cites W2885109269 @default.
- W4285743376 cites W2948930298 @default.
- W4285743376 cites W2963072799 @default.
- W4285743376 cites W2980007004 @default.
- W4285743376 cites W3003118458 @default.
- W4285743376 cites W3036977507 @default.
- W4285743376 cites W3093743078 @default.
- W4285743376 cites W3110776361 @default.
- W4285743376 cites W3173298378 @default.
- W4285743376 cites W3197942682 @default.
- W4285743376 cites W4238292505 @default.
- W4285743376 cites W4249102227 @default.
- W4285743376 doi "https://doi.org/10.1140/epjd/s10053-022-00430-6" @default.
- W4285743376 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/35782906" @default.
- W4285743376 hasPublicationYear "2022" @default.
- W4285743376 type Work @default.
- W4285743376 citedByCount "2" @default.
- W4285743376 countsByYear W42857433762022 @default.
- W4285743376 countsByYear W42857433762023 @default.
- W4285743376 crossrefType "journal-article" @default.
- W4285743376 hasAuthorship W4285743376A5001069974 @default.
- W4285743376 hasAuthorship W4285743376A5009223920 @default.
- W4285743376 hasAuthorship W4285743376A5014009587 @default.
- W4285743376 hasAuthorship W4285743376A5023741536 @default.
- W4285743376 hasAuthorship W4285743376A5027797652 @default.
- W4285743376 hasAuthorship W4285743376A5042304241 @default.
- W4285743376 hasAuthorship W4285743376A5049936709 @default.
- W4285743376 hasAuthorship W4285743376A5056949461 @default.
- W4285743376 hasAuthorship W4285743376A5057184832 @default.
- W4285743376 hasAuthorship W4285743376A5087798025 @default.
- W4285743376 hasBestOaLocation W42857433761 @default.
- W4285743376 hasConcept C102931765 @default.
- W4285743376 hasConcept C103862110 @default.
- W4285743376 hasConcept C105795698 @default.
- W4285743376 hasConcept C120665830 @default.
- W4285743376 hasConcept C121332964 @default.
- W4285743376 hasConcept C145148216 @default.
- W4285743376 hasConcept C147789679 @default.
- W4285743376 hasConcept C155672457 @default.
- W4285743376 hasConcept C158355884 @default.
- W4285743376 hasConcept C159467904 @default.
- W4285743376 hasConcept C171250308 @default.
- W4285743376 hasConcept C178790620 @default.
- W4285743376 hasConcept C185592680 @default.
- W4285743376 hasConcept C192562407 @default.
- W4285743376 hasConcept C19499675 @default.
- W4285743376 hasConcept C2780358262 @default.
- W4285743376 hasConcept C2780471494 @default.
- W4285743376 hasConcept C32909587 @default.
- W4285743376 hasConcept C33923547 @default.
- W4285743376 hasConcept C62520636 @default.
- W4285743376 hasConcept C82706917 @default.
- W4285743376 hasConceptScore W4285743376C102931765 @default.
- W4285743376 hasConceptScore W4285743376C103862110 @default.
- W4285743376 hasConceptScore W4285743376C105795698 @default.
- W4285743376 hasConceptScore W4285743376C120665830 @default.
- W4285743376 hasConceptScore W4285743376C121332964 @default.
- W4285743376 hasConceptScore W4285743376C145148216 @default.
- W4285743376 hasConceptScore W4285743376C147789679 @default.
- W4285743376 hasConceptScore W4285743376C155672457 @default.
- W4285743376 hasConceptScore W4285743376C158355884 @default.
- W4285743376 hasConceptScore W4285743376C159467904 @default.
- W4285743376 hasConceptScore W4285743376C171250308 @default.
- W4285743376 hasConceptScore W4285743376C178790620 @default.
- W4285743376 hasConceptScore W4285743376C185592680 @default.
- W4285743376 hasConceptScore W4285743376C192562407 @default.
- W4285743376 hasConceptScore W4285743376C19499675 @default.
- W4285743376 hasConceptScore W4285743376C2780358262 @default.