FRINK Linked Data Fragments server

Matches in SemOpenAlex for { <https://semopenalex.org/work/W4285793359> ?p ?o ?g. }

• W4285793359 abstract "Single-atom catalysts (SACs) as the new frontier in heterogeneous catalysis have attracted increasing attention. However, the rational design of SACs with high catalytic activities for specified reactions still remains challenging. Herein, we report the rational design of a Pd1-PdNPs synergistic structure on 2,6-pyridinedicarbonitrile-derived covalent triazine framework (CTF) as an efficient active site for CO2 hydrogenation to formate under ambient conditions. Compared with the catalysts mainly comprising Pd1 and PdNPs, this hybrid catalyst presented significantly improved catalytic activity. By regulating the ratio of Pd1 to PdNPs, we obtained the optimal catalytic activity with a formate formation rate of 3.66 molHCOOM·molPd-1·h-1 under ambient conditions (30°C, 0.1 MPa). Moreover, as a heterogeneous catalyst, this hybrid catalyst is easily recovered and exhibits about a 20% decrease in the catalytic activity after five cycles. These findings are significant in elucidating new rational design principles for CO2 hydrogenation catalysts with superior activity and may open up the possibilities of converting CO2 under ambient conditions." @default.
• W4285793359 created "2022-07-19" @default.
• W4285793359 creator A5004771945 @default.
• W4285793359 creator A5010444377 @default.
• W4285793359 creator A5017306873 @default.
• W4285793359 creator A5027584684 @default.
• W4285793359 creator A5030566798 @default.
• W4285793359 creator A5055466064 @default.
• W4285793359 creator A5078588014 @default.
• W4285793359 creator A5079909263 @default.
• W4285793359 creator A5083172885 @default.
• W4285793359 creator A5083228843 @default.
• W4285793359 date "2022-07-19" @default.
• W4285793359 modified "2023-10-15" @default.
• W4285793359 title "Rational Design of Synergistic Structure Between Single-Atoms and Nanoparticles for CO2 Hydrogenation to Formate Under Ambient Conditions" @default.
• W4285793359 cites W1853374276 @default.
• W4285793359 cites W1966182479 @default.
• W4285793359 cites W1970127494 @default.
• W4285793359 cites W1979371521 @default.
• W4285793359 cites W1988320534 @default.
• W4285793359 cites W1992173555 @default.
• W4285793359 cites W2003193361 @default.
• W4285793359 cites W2007395042 @default.
• W4285793359 cites W2036113194 @default.
• W4285793359 cites W2046412723 @default.
• W4285793359 cites W2077661812 @default.
• W4285793359 cites W2083222334 @default.
• W4285793359 cites W2104015519 @default.
• W4285793359 cites W2107890759 @default.
• W4285793359 cites W2122427541 @default.
• W4285793359 cites W2134716155 @default.
• W4285793359 cites W2150195378 @default.
• W4285793359 cites W2356997838 @default.
• W4285793359 cites W2474398724 @default.
• W4285793359 cites W2565870685 @default.
• W4285793359 cites W2725648806 @default.
• W4285793359 cites W2768004292 @default.
• W4285793359 cites W2789772982 @default.
• W4285793359 cites W2800597554 @default.
• W4285793359 cites W2803427589 @default.
• W4285793359 cites W2903365446 @default.
• W4285793359 cites W2934429683 @default.
• W4285793359 cites W2995970219 @default.
• W4285793359 cites W3009222120 @default.
• W4285793359 cites W3009430568 @default.
• W4285793359 cites W4200409645 @default.
• W4285793359 doi "https://doi.org/10.3389/fchem.2022.957412" @default.
• W4285793359 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/35928210" @default.
• W4285793359 hasPublicationYear "2022" @default.
• W4285793359 type Work @default.
• W4285793359 citedByCount "2" @default.
• W4285793359 countsByYear W42857933592023 @default.
• W4285793359 crossrefType "journal-article" @default.
• W4285793359 hasAuthorship W4285793359A5004771945 @default.
• W4285793359 hasAuthorship W4285793359A5010444377 @default.
• W4285793359 hasAuthorship W4285793359A5017306873 @default.
• W4285793359 hasAuthorship W4285793359A5027584684 @default.
• W4285793359 hasAuthorship W4285793359A5030566798 @default.
• W4285793359 hasAuthorship W4285793359A5055466064 @default.
• W4285793359 hasAuthorship W4285793359A5078588014 @default.
• W4285793359 hasAuthorship W4285793359A5079909263 @default.
• W4285793359 hasAuthorship W4285793359A5083172885 @default.
• W4285793359 hasAuthorship W4285793359A5083228843 @default.
• W4285793359 hasBestOaLocation W42857933591 @default.
• W4285793359 hasConcept C127413603 @default.
• W4285793359 hasConcept C155672457 @default.
• W4285793359 hasConcept C161790260 @default.
• W4285793359 hasConcept C171250308 @default.
• W4285793359 hasConcept C178790620 @default.
• W4285793359 hasConcept C180577832 @default.
• W4285793359 hasConcept C185592680 @default.
• W4285793359 hasConcept C192562407 @default.
• W4285793359 hasConcept C21951064 @default.
• W4285793359 hasConcept C2780178953 @default.
• W4285793359 hasConcept C42360764 @default.
• W4285793359 hasConcept C53105671 @default.
• W4285793359 hasConceptScore W4285793359C127413603 @default.
• W4285793359 hasConceptScore W4285793359C155672457 @default.
• W4285793359 hasConceptScore W4285793359C161790260 @default.
• W4285793359 hasConceptScore W4285793359C171250308 @default.
• W4285793359 hasConceptScore W4285793359C178790620 @default.
• W4285793359 hasConceptScore W4285793359C180577832 @default.
• W4285793359 hasConceptScore W4285793359C185592680 @default.
• W4285793359 hasConceptScore W4285793359C192562407 @default.
• W4285793359 hasConceptScore W4285793359C21951064 @default.
• W4285793359 hasConceptScore W4285793359C2780178953 @default.
• W4285793359 hasConceptScore W4285793359C42360764 @default.
• W4285793359 hasConceptScore W4285793359C53105671 @default.
• W4285793359 hasFunder F4320321001 @default.
• W4285793359 hasFunder F4320324174 @default.
• W4285793359 hasFunder F4320335777 @default.
• W4285793359 hasLocation W42857933591 @default.
• W4285793359 hasLocation W42857933592 @default.
• W4285793359 hasLocation W42857933593 @default.
• W4285793359 hasLocation W42857933594 @default.
• W4285793359 hasOpenAccess W4285793359 @default.
• W4285793359 hasPrimaryLocation W42857933591 @default.
• W4285793359 hasRelatedWork W117391990 @default.
• W4285793359 hasRelatedWork W1624343457 @default.
• W4285793359 hasRelatedWork W1855652426 @default.

• next