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- W4285801053 abstract "Abstract The phase evolutions in sodium hydroxide and sodium silicate–activated slag cements upon sulfate salt attack were investigated via thermodynamic modeling. The effects of different sulfate salts (i.e., Na 2 SO 4 and MgSO 4 ) and slag compositions were studied. In thermodynamic modeling, a solid solution model, that is, MgAl–SO 4 –LDH_ss, was proposed to describe the sulfate‐intercalated hydrotalcite. The modeling results were presented and discussed in comparison with experimental observations. Upon sulfate salt attack, ettringite, gypsum, sulfate‐intercalated hydrotalcite, magnesium silicate hydrate, and so on were predicted to form. By quantitatively evaluating the composition change of C–(N–)A–S–H gel, solid phase expansion, and alteration in pore solution chemistry, it was found that magnesium sulfate induced severer degradation of alkali‐activated slag cements compared to sodium sulfate. Upon sulfate salt attack with a fixed sulfate concentration, the ideal outcome shows that the slag with lower Al 2 O 3 content not only gave a larger content of C–(N–)A–S–H gel but also caused the reduced decalcification and dealumination of C–(N–)A–S–H gel and solid phase expansion." @default.
- W4285801053 created "2022-07-19" @default.
- W4285801053 creator A5009302091 @default.
- W4285801053 date "2022-07-29" @default.
- W4285801053 modified "2023-09-26" @default.
- W4285801053 title "Thermodynamic modeling of the phase evolution in alkali‐activated slag cements with sulfate salt exposure" @default.
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- W4285801053 doi "https://doi.org/10.1111/jace.18661" @default.
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