Matches in SemOpenAlex for { <https://semopenalex.org/work/W4286268132> ?p ?o ?g. }
- W4286268132 endingPage "138208" @default.
- W4286268132 startingPage "138208" @default.
- W4286268132 abstract "All-solid-state lithium-sulfur batteries (ALSBs) using poly(ethylene oxide) (PEO)-based composite solid-state electrolytes (CSEs) are regarded as one of potential high energy storage devices; however, they still face two core problems of polysulfide shuttle and lithium dendrite during long cycle. Herein, based on a passive-type strategy, magnesium bis(trifluoromethylsulphonyl)imide [Mg(TFSI)2] as a novel functional additive of the PEO-Li6.5La3Zr1.5Ta0.5O12 (PEO-LLZTO)-based CSE, has been proved to be successful on both retarding polysulfide species shuttle and stabilizing lithium anode. Study results show that magnesium polysulfide precipitate, formed on the interface between the S/C cathode and CSE, can hinder the shuttle of diffluent lithium polysulfide; and meanwhile, a robust LixMg layer generated on the surface of lithium anode can suppress the formation of dendrite. As a consequence, the Mg(TFSI)2 additive-functionalized PEO-LLZTO CSE obviously prompts a critical current density up to 1.0 mA cm−2 from 0.6 mA cm−2 of the sole PEO-LLZTO CSE, and maintains very stable cycling over 500 h at 0.2 mA cm−2 for a symmetric cell. Furthermore, the ALSB with the Mg(TFSI)2 additive-functionalized PEO-LLZTO CSE delivers robust cycle performances, with specific capacities of 877 mAh g−1 at 0.1C (1C = 1675 mA g−1) after 50 cycles (capacity retention ratio of 100 %) and 331 mAh g−1 at 0.5C over 300 cycles (capacity retention ratio of 94.1 %) under 50 °C. This work provides a realistic reference in designing novel additives to ameliorate the electrode–electrolyte interfaces for stabilizing ALSB." @default.
- W4286268132 created "2022-07-21" @default.
- W4286268132 creator A5015603159 @default.
- W4286268132 creator A5019477992 @default.
- W4286268132 creator A5056165846 @default.
- W4286268132 creator A5062520365 @default.
- W4286268132 creator A5086300353 @default.
- W4286268132 date "2022-12-01" @default.
- W4286268132 modified "2023-10-17" @default.
- W4286268132 title "A functional additive to in-situ construct stable cathode and anode interfaces for all-solid-state lithium-sulfur batteries" @default.
- W4286268132 cites W2065077785 @default.
- W4286268132 cites W2171394752 @default.
- W4286268132 cites W2313604584 @default.
- W4286268132 cites W2324000835 @default.
- W4286268132 cites W2482083820 @default.
- W4286268132 cites W2490292921 @default.
- W4286268132 cites W2605190567 @default.
- W4286268132 cites W2747027649 @default.
- W4286268132 cites W2789638551 @default.
- W4286268132 cites W2793336898 @default.
- W4286268132 cites W2887482625 @default.
- W4286268132 cites W2898341143 @default.
- W4286268132 cites W2913959819 @default.
- W4286268132 cites W2945149024 @default.
- W4286268132 cites W2947611771 @default.
- W4286268132 cites W2948222308 @default.
- W4286268132 cites W2969387578 @default.
- W4286268132 cites W2969809408 @default.
- W4286268132 cites W2991243995 @default.
- W4286268132 cites W3004390254 @default.
- W4286268132 cites W3010031341 @default.
- W4286268132 cites W3011688209 @default.
- W4286268132 cites W3022794757 @default.
- W4286268132 cites W3024529292 @default.
- W4286268132 cites W3037180228 @default.
- W4286268132 cites W3040594568 @default.
- W4286268132 cites W3094784679 @default.
- W4286268132 cites W3111453967 @default.
- W4286268132 cites W3127348006 @default.
- W4286268132 cites W3129499345 @default.
- W4286268132 cites W3137365443 @default.
- W4286268132 cites W3152129813 @default.
- W4286268132 cites W3158251771 @default.
- W4286268132 cites W3168637836 @default.
- W4286268132 cites W3174041921 @default.
- W4286268132 cites W3184195056 @default.
- W4286268132 cites W3186831656 @default.
- W4286268132 cites W3196454815 @default.
- W4286268132 cites W3205269758 @default.
- W4286268132 cites W3209558903 @default.
- W4286268132 cites W3216216817 @default.
- W4286268132 cites W3216755742 @default.
- W4286268132 cites W4200460363 @default.
- W4286268132 cites W4205954702 @default.
- W4286268132 cites W4211108632 @default.
- W4286268132 cites W4212775077 @default.
- W4286268132 cites W4214914276 @default.
- W4286268132 cites W4223953941 @default.
- W4286268132 cites W4285185387 @default.
- W4286268132 doi "https://doi.org/10.1016/j.cej.2022.138208" @default.
- W4286268132 hasPublicationYear "2022" @default.
- W4286268132 type Work @default.
- W4286268132 citedByCount "8" @default.
- W4286268132 countsByYear W42862681322022 @default.
- W4286268132 countsByYear W42862681322023 @default.
- W4286268132 crossrefType "journal-article" @default.
- W4286268132 hasAuthorship W4286268132A5015603159 @default.
- W4286268132 hasAuthorship W4286268132A5019477992 @default.
- W4286268132 hasAuthorship W4286268132A5056165846 @default.
- W4286268132 hasAuthorship W4286268132A5062520365 @default.
- W4286268132 hasAuthorship W4286268132A5086300353 @default.
- W4286268132 hasConcept C127413603 @default.
- W4286268132 hasConcept C134018914 @default.
- W4286268132 hasConcept C147789679 @default.
- W4286268132 hasConcept C17525397 @default.
- W4286268132 hasConcept C185592680 @default.
- W4286268132 hasConcept C191897082 @default.
- W4286268132 hasConcept C192562407 @default.
- W4286268132 hasConcept C2524010 @default.
- W4286268132 hasConcept C2777379467 @default.
- W4286268132 hasConcept C2778541603 @default.
- W4286268132 hasConcept C33923547 @default.
- W4286268132 hasConcept C42360764 @default.
- W4286268132 hasConcept C49110097 @default.
- W4286268132 hasConcept C518881349 @default.
- W4286268132 hasConcept C543218039 @default.
- W4286268132 hasConcept C68801617 @default.
- W4286268132 hasConcept C71924100 @default.
- W4286268132 hasConcept C84248122 @default.
- W4286268132 hasConcept C89395315 @default.
- W4286268132 hasConceptScore W4286268132C127413603 @default.
- W4286268132 hasConceptScore W4286268132C134018914 @default.
- W4286268132 hasConceptScore W4286268132C147789679 @default.
- W4286268132 hasConceptScore W4286268132C17525397 @default.
- W4286268132 hasConceptScore W4286268132C185592680 @default.
- W4286268132 hasConceptScore W4286268132C191897082 @default.
- W4286268132 hasConceptScore W4286268132C192562407 @default.
- W4286268132 hasConceptScore W4286268132C2524010 @default.