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- W4286322019 abstract "β-Thiolated-α-arylated ketones are perversive in bioactive molecules and serve as potential bidentate ligands for catalysis. Herein, a straightforward protocol to access β-thiolated ketones from aldehydes, alkenes, and disulfides enabled by the combination of photocatalysis and N-heterocyclic carbene catalysis is reported. The sequential radical addition to alkenes and subsequent radical-radical coupling cascade process simultaneously forge C-S and C-C bonds. The mild conditions allow for radical relay coupling with a broad functional group tolerance." @default.
- W4286322019 created "2022-07-21" @default.
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- W4286322019 date "2022-07-21" @default.
- W4286322019 modified "2023-10-15" @default.
- W4286322019 title "Synthesis of β-Thiolated-α-arylated Ketones Enabled by Photoredox and <i>N</i>-Heterocyclic Carbene-Catalyzed Radical Relay of Alkenes with Disulfides and Aldehydes" @default.
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- W4286322019 doi "https://doi.org/10.1021/acs.orglett.2c01915" @default.
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