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- W4286436600 abstract "The large-scale fabrication of high-quality carbon nanotube (CNT) arrays with highly uniform orientation is challenging due to the relatively low carbon conversion rate. Herein, a plasma-modified flaky FeSiAl (FSA) catalyst was developed for the high- efficiency conversion from acetylene to CNT arrays by catalytic chemical vapor deposition (CCVD). The surface nanoparticles of plasma-modified FSA were refined and oxidized, resulting in an increase in the catalytic active oxides as well as a high carbon conversion rate up to ~97.2%. The growth mechanism analysis confirmed the base-symmetric growth mode of CNT arrays and the maximum theoretical CNT array yield was predicted to be ~8.20 g when using 0.5 g plasma-modified FSA catalysts. The apparent activation energy of CNT arrays was calculated to be ~53.17 kJ/mol, indicating the coexistence of surface diffusion on the catalysts and step-edge diffusion at the graphene-catalyst interface. This work provides a highly efficient methodology for the low-cost and large-scale production of CNT arrays with potential application in the field of high-performance energy storage." @default.
- W4286436600 created "2022-07-22" @default.
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- W4286436600 date "2022-11-01" @default.
- W4286436600 modified "2023-10-03" @default.
- W4286436600 title "Plasma-modified flaky FeSiAl alloy for efficient growth of carbon nanotube arrays with high carbon conversion rate" @default.
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- W4286436600 doi "https://doi.org/10.1016/j.jallcom.2022.166453" @default.
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