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• W4286567111 endingPage "138236" @default.
• W4286567111 startingPage "138236" @default.
• W4286567111 abstract "Garnet-based solid-state electrolytes (SSEs) have received great attention due to their high ionic conductivity and superior chemical/electrochemical stabilities. However, the high interfacial resistance induced by the poor wettability of the Li/SSEs interface and the resulting Li dendrite penetration severely hinder the practical application of garnet-based all-solid-state Li metal batteries (ASSLMBs). Herein, we explore a low-cost and facile molten salt coating method to uniformly coat an ultrathin SnF2 film on the surface of garnet-type Li6.4La3Zr1.4Ta0.6O12 (LLZTO) SSEs. After lithiation at elevated temperature, the SnF2 film is in-situ transformed into hybrid interphase composed of LiF and Li22Sn5. Highly lithiophilic Li22Sn5 alloy provides intimate contact between Li and LLZTO, while electron-blocking LiF prevents Li deposition within LLZTO. Therefore, assembled Li|SnF2-coated LLZTO|Li cells can cycle stably at 0.3 mA cm−2 over 1000 h and achieve a high critical current density of 1.0 mA cm−2. Moreover, the Li|SnF2-coated LLZTO|LiFePO4 full cells exhibit superior cycling (88.9 % capacity retention over 400 cycles at 0.5C) and rate performance. Notably, the proposed salt coating strategy endows an extended degree of freedom for functional interfacial design and potential for large-scale application, given the abundance of salt species and low cost and complexity of heating treatment, respectively." @default.
• W4286567111 created "2022-07-22" @default.
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• W4286567111 date "2022-12-01" @default.
• W4286567111 modified "2023-10-16" @default.
• W4286567111 title "Low-cost molten salt coating enabling robust Li/garnet interface for dendrite-free all-solid-state lithium batteries" @default.
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• W4286567111 doi "https://doi.org/10.1016/j.cej.2022.138236" @default.
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