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- W4286799963 abstract "Hot carriers produced from the decay of localized surface plasmons in metallic nanoparticles are intensely studied because of their optoelectronic, photovoltaic and photocatalytic applications. From a classical perspective, plasmons are coherent oscillations of the electrons in the nanoparticle, but their quantized nature comes to the fore in the novel field of quantum plasmonics. In this work, we introduce a quantum-mechanical material-specific approach for describing the decay of single quantized plasmons into hot electrons and holes. We find that hot carrier generation rates differ significantly from semiclassical predictions. We also investigate the decay of excitations without plasmonic character and show that their hot carrier rates are comparable to those from the decay of plasmonic excitations for small nanoparticles. Our study provides a rigorous and general foundation for further development of plasmonic hot carrier studies in the plasmonic regime required for the design of ultrasmall devices." @default.
- W4286799963 created "2022-07-24" @default.
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- W4286799963 date "2019-04-07" @default.
- W4286799963 modified "2023-10-01" @default.
- W4286799963 title "Single plasmon hot carrier generation in metallic nanoparticles" @default.
- W4286799963 doi "https://doi.org/10.48550/arxiv.1904.03697" @default.
- W4286799963 hasPublicationYear "2019" @default.
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