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• W4287735701 abstract "Abstract Porous Organic Cages (POCs) with tunable tailoring chemistry properties and polymer‐like processing conditions are of great potential for molecular selective membranes, but it remains challenging in the assembly of high crystalline POCs with regular nanochannels for effective molecular sieving. Here we report an electrostatic‐induced crystal‐rearrangement strategy for the design of a POC membrane with heterostructure. Due to electrostatic attraction, ionic liquid molecules induced cage molecules to rearrange into a sub‐10 nm uniform and defect‐free crystal layer, which displayed competitive CO 2 separation performance. The optimized hetero‐structured membrane exhibited an attractive CO 2 /N 2 separation selectivity of over 130, which was superior to the state‐of‐the‐art membranes, accompanied with excellent long‐term and thermal shock stability. This strategy provides a new inspiration for the preparation of crystal‐rearranged membranes with regular channels for gas molecule sieving." @default.
• W4287735701 created "2022-07-26" @default.
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• W4287735701 date "2022-06-15" @default.
• W4287735701 modified "2023-10-17" @default.
• W4287735701 title "Electrostatic‐Induced Crystal‐Rearrangement of Porous Organic Cage Membrane for CO ₂ Capture" @default.
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• W4287735701 doi "https://doi.org/10.1002/ange.202205481" @default.
• W4287735701 hasPublicationYear "2022" @default.
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