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- W4287881779 abstract "Atomic-level structure characterization is central to the science and engineering of materials. However, the crystal structure determination of magic-sized nanoclusters (MSCs), typical nuclei of the semiconductor nanocrystals, is impeded by challenges in obtaining phase-pure MSCs. Herein, we report on the synthesis and X-ray crystal structure of ∼0.9-nanometer-sized 27-atom semiconductor MSC, Cd14Se13. Its structure has a central Se atom encapsulated by a Cd14Se12 cage with an adamantane-like CdSe arrangement. Two chloride ions released in situ from the dichloromethane solvent stabilize and linearly self-assemble the clusters. The formation and growth pathways of Cd14Se13 clusters provide vital insights into the size-structure-property relationships in MSCs. Furthermore, potential sites for magnetic dopants are identified in Cd14Se13 MSC, enabling research on atomically precise dilute magnetic semiconductors." @default.
- W4287881779 created "2022-07-26" @default.
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- W4287881779 date "2022-11-01" @default.
- W4287881779 modified "2023-10-17" @default.
- W4287881779 title "Structure of a subnanometer-sized semiconductor Cd14Se13 cluster" @default.
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- W4287881779 doi "https://doi.org/10.1016/j.chempr.2022.06.025" @default.
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