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• W4288038891 abstract "A palladium-catalyzed deuterated formylation of aryl sulfonium salts is prepared conveniently from readily available arenes, which enables the expedient synthesis of a series of structurally diverse C-1 deuterated aldehydes with 96%–99% deuterium incorporation. The easy to handle and cost-effective DCOONa provides a deuterium source, which can be introduced onto the formyl units with excellent selectivity under the palladium-catalytic redox neutral conditions. This catalytic route can accomplish the direct late-stage C–H functionalization of bioactive molecules and natural product derivatives assisted by C (sp2)–H thianthrenation. Moreover, on the basis of this practical approach, several deuterated drugs and analogues could be prepared with excellent levels of deuterium incorporation." @default.
• W4288038891 created "2022-07-27" @default.
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• W4288038891 date "2022-07-26" @default.
• W4288038891 modified "2023-10-13" @default.
• W4288038891 title "Palladium-Catalyzed Synthesis of C-1 Deuterated Aldehydes from (Hetero) Arenes Mediated by C (sp²)–H Thianthrenation" @default.
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• W4288038891 doi "https://doi.org/10.1021/acs.orglett.2c02328" @default.
• W4288038891 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/35880900" @default.
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