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• W4288045126 abstract "Silicon nanoparticles (Si NPs) are potential anode materials for next-generation lithium-ion batteries due to their natural abundance, low discharge potential, and high theoretical capacity. Carbon coating improves the capacity of the Si NPs, protects them from disintegration during the lithiation/delithiation process, and provides an additional conductive matrix. Surface modification as a tool leading to capacity enhancement in carbon-coated Si NPs has rarely been explored. It is a straightforward process that involves the surface functionalization of carbon-coated Si NPs (Si-C) with the oxidizing acidic mixture. The surface-treated Si-C functionalized with carboxyl and hydroxyl groups in excess on the carbon surface of Si-C NPs. As a result of surface modification, the acid-treated Si-C (Si-C-AT) displayed a higher reversible capacity of 1575 mA h g−1 after 200 cycles compared to the Si-C (1261 mA h g−1) and bare Si (961 mA h g−1). This high capacity of Si-C-AT is a cumulative outcome of the functional groups and the disordered structure of the carbon shell. The functional groups act as lithophilic sites, and the disordered carbon shell facilitates the insertion-desertion of lithium ions. The simple surface modification strategy proposed in the present study significantly enhances the cyclability of the Si-C-AT NPs and has great potential for application in carbon-coated materials for lithium-ion batteries." @default.
• W4288045126 created "2022-07-27" @default.
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• W4288045126 date "2022-11-01" @default.
• W4288045126 modified "2023-10-17" @default.
• W4288045126 title "Performance enhancement of carbon-coated Si nanoparticles for lithium-ion batteries through the generation of lithophilic sites by a simple oxidation process" @default.
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• W4288045126 doi "https://doi.org/10.1016/j.apsusc.2022.154361" @default.
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