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• W4288052302 abstract "Abstract The cathode material is critical to the yield of hydrogen peroxide (H2O2) and electro-Fenton (EF) performance. In this work, bismuth oxychloride (BiOCl) as one of the representatives of ternary oxides was grown in situ on carbon felt (CF) through a simple solvothermal method and employed directly as a self-standing cathode for the EF degradation of the target contaminant tetracycline (TC). TC can be almost completely degraded, up to 95% in 90 min under the heterogeneous EF process. The characterizations demonstrated that the BiOCl/CF electrode exhibited excellent conductivity due to CF as the supporting carbon material with a 3D network structure; meanwhile, this hybrid electrode also possessed abundant active sites attributed to the decorated BiOCl having rich oxygen defects. Finally, the rational reaction mechanism of TC was also elucidated by the X-ray photoelectron spectroscopy (XPS) spectrum, free radical quenching experiments and electron paramagnetic resonance (EPR) spectra, in which hydroxyl radicals () were considered as the dominant active oxidants and BiOCl had a synergistic effect on in-situ generation and decomposition of H2O2. HIGHLIGHTS A BiOCl/CF composite electrode was prepared via a simple solvothermal method. Oxygen defects enriched BiOCl and bare carbon felt cathode had a synergistic effect on H2O2 production. Lattice oxygen reduced Bi3+ to Bi0, facilitating the formation of by in situ reaction of hydrogen peroxide with Bi0. was the main radical in catalytic degradation of tetracycline." @default.
• W4288052302 created "2022-07-28" @default.
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• W4288052302 date "2022-07-27" @default.
• W4288052302 modified "2023-09-30" @default.
• W4288052302 title "Enhanced electro-Fenton degradation of tetracycline in aqueous solution using a self-supported BiOCl/CF cathode" @default.
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• W4288052302 doi "https://doi.org/10.2166/wst.2022.230" @default.
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