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- W4288383989 abstract "Self-assembly and on-surface synthesis are vital strategies used for fabricating surface-confined 1D or 2D supramolecular nanoarchitectures with atomic precision. In many systems, the resulting structure is determined by the kinetics of the processes involved, i.e., reaction rate, on-surface diffusion, nucleation, and growth, all of which are typically governed by temperature. However, other external factors have been only scarcely harnessed to control the on-surface chemical reaction kinetics and self-assembly. Here, we show that a low-energy electron beam can be used to steer chemical reaction kinetics and induce the growth of molecular phases unattainable by thermal annealing. The electron beam provides a well-controlled means of promoting the elementary reaction step, i.e., deprotonation of carboxyl groups. The reaction rate increases with the increasing electron beam energy beyond the threshold energy of 6 eV. Our results offer the novel prospect of controlling self-assembly, enhancing the rate of reaction steps selectively, and thus altering the kinetic rate hierarchy." @default.
- W4288383989 created "2022-07-29" @default.
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- W4288383989 date "2022-10-01" @default.
- W4288383989 modified "2023-09-30" @default.
- W4288383989 title "Kinetic control of self-assembly using a low-energy electron beam" @default.
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- W4288383989 doi "https://doi.org/10.1016/j.apsusc.2022.154106" @default.
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