Matches in SemOpenAlex for { <https://semopenalex.org/work/W4288385628> ?p ?o ?g. }
- W4288385628 abstract "Abstract The industrialization of lithium–sulfur (Li–S) batteries is simultaneously impeded by the shuttle effect of lithium polysulfides and dendrites growth on lithium anode. To address both issues, a novel sulfiphilic and lithiophilic interlayer of Mo 2 N quantum dots decorated N‐doped graphene‐nanosheet (Mo 2 N@NG) are presented on polypropylene separator via a facile scalable method. Benefiting from the strong chemisorption ability, eminent electrocatalysis for LiPSs, and high chemical affinity with lithium‐ion (Li + ), Mo 2 N@NG can efficiently catalyze the rapid transformation of LiPSs and induce uniform deposition of Li + . Theoretical calculation and in situ Raman synergistically elucidate the inhibition of shuttle effect and alleviation of dendrite growth. As a result, the assembled Li–S cell with Mo 2 N@NG/PP separator exhibits remarkable rate performance (860.2 mA h g –1 at 4 C), good cycling stability (0.039% capacity decay per cycle after 800 cycles at 2 C), a high areal capacity of 3.89 mA h cm –2 of Li–S pouch cell (4.5 mg cm –2 and 6 µL mg –1 at 0.2 C), and steady performance in protecting the lithium anode (at 5 mA cm –2 for 1500 h). This present strategy of quantum dots in a hybrid framework has great potential to be generalized to other transition metal‐based catalysts for advanced Li–S batteries." @default.
- W4288385628 created "2022-07-29" @default.
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- W4288385628 date "2022-07-28" @default.
- W4288385628 modified "2023-10-18" @default.
- W4288385628 title "Mo<sub>2</sub>N Quantum Dots Decorated N‐Doped Graphene Nanosheets as Dual‐Functional Interlayer for Dendrite‐Free and Shuttle‐Free Lithium‐Sulfur Batteries" @default.
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- W4288385628 doi "https://doi.org/10.1002/adfm.202206113" @default.
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