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• W4288702954 abstract "Designing anode materials with high lithium specific capacity is crucial to the development of high energy-density lithium ion batteries. Herein, a distinctive lithium growth mechanism, namely, the restricted multilayered growth for lithium, and a strategy for lithium storage are proposed to achieve the balance between the ultra-high specific capacity and the need to avert uncontrolled dendritic growth of lithium. In particular, based on first-principles computation, we show that the Al2C monolayer with planar tetracoordinate carbon structure can be an ideal platform for realizing the restricted multilayered growth mechanism as a 2D anode material. Furthermore, the Al2C monolayer exhibits ultra-high specific capacity of lithium of 4059 mAh/g, yet with a low dif-fusion barrier of 0.039-0.17 eV as well as low open circuit voltage in the range of 0.002-0.34 V. These novel properties endow the Al2C monolayer a promising anode material for future lithium ion batteries. Our study offers a new way to design promising 2D anode materials with high specific capacity, fast lithium-ion diffusion, and safe lithium storage mechanism." @default.
• W4288702954 created "2022-07-30" @default.
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• W4288702954 date "2022-07-29" @default.
• W4288702954 modified "2023-10-15" @default.
• W4288702954 title "Ultrahigh Lithium Storage Capacity of Al₂C Monolayer in a Restricted Multilayered Growth Mechanism" @default.
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• W4288702954 doi "https://doi.org/10.1021/acsami.2c07980" @default.
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