FRINK Linked Data Fragments server

Matches in SemOpenAlex for { <https://semopenalex.org/work/W4288712745> ?p ?o ?g. }

• W4288712745 endingPage "1658" @default.
• W4288712745 startingPage "1653" @default.
• W4288712745 abstract "Lithium–Sulfur (Li–S) batteries are one of the most promising next-generation batteries due to their ultrahigh energy density up to 500 W h kg–1. However, despite the steady progress during the last several decades, there have been significant challenges for practical applications and commercialization. One of the major issues is controlling the lithium polysulfide (LiPS) shuttling process, which causes premature cell failure. To better understand the mechanism of the LiPS shuttling chemistry, a qualitative and quantitative analysis on polysulfide species in Li–S cell has profound significance for realizing highly efficient sulfur electrochemistry. Here we report a qualitative determination of the derivatized polysulfides in the electrolyte of a custom-made Li–S pouch cell with a high-resolution liquid chromatography-atmospheric pressure chemical ionization tandem mass spectrometry method for the first time. The ionization efficiency of the methylated polysulfides was affected by the tune parameters such as the corona discharge current, the vaporizer temperature, and the source capillary temperature. It was found that the source capillary temperature was the dominant parameter to increase the peak intensity of CH3S7– ion, which was the smallest peak in the spectrum. An unusual and unique ionization pattern for methylated polysulfides detected in atmospheric pressure chemical ionization negative mode was elucidated by using first-principles calculations." @default.
• W4288712745 created "2022-07-30" @default.
• W4288712745 creator A5011972457 @default.
• W4288712745 creator A5019770299 @default.
• W4288712745 creator A5033119802 @default.
• W4288712745 creator A5036433151 @default.
• W4288712745 creator A5069278408 @default.
• W4288712745 creator A5073114604 @default.
• W4288712745 creator A5076661275 @default.
• W4288712745 date "2022-07-29" @default.
• W4288712745 modified "2023-09-27" @default.
• W4288712745 title "Qualitative Determination of Polysulfide Species in a Lithium–Sulfur Battery by HR-LC-APCI-MSⁿ with One-Step Derivatization" @default.
• W4288712745 cites W1748242565 @default.
• W4288712745 cites W1943504659 @default.
• W4288712745 cites W1970905334 @default.
• W4288712745 cites W1977928242 @default.
• W4288712745 cites W1978880154 @default.
• W4288712745 cites W2010168042 @default.
• W4288712745 cites W2023271753 @default.
• W4288712745 cites W2057899803 @default.
• W4288712745 cites W2068601436 @default.
• W4288712745 cites W2070598587 @default.
• W4288712745 cites W2080630504 @default.
• W4288712745 cites W2083164683 @default.
• W4288712745 cites W2095940702 @default.
• W4288712745 cites W2110826247 @default.
• W4288712745 cites W2125658152 @default.
• W4288712745 cites W2135735962 @default.
• W4288712745 cites W2143981217 @default.
• W4288712745 cites W2314434099 @default.
• W4288712745 cites W2316548329 @default.
• W4288712745 cites W2323147066 @default.
• W4288712745 cites W2324000835 @default.
• W4288712745 cites W2509056915 @default.
• W4288712745 cites W2593650871 @default.
• W4288712745 cites W2612700249 @default.
• W4288712745 cites W2774119270 @default.
• W4288712745 cites W2789705881 @default.
• W4288712745 cites W2791810492 @default.
• W4288712745 cites W2884003303 @default.
• W4288712745 cites W2890815815 @default.
• W4288712745 cites W2948196514 @default.
• W4288712745 cites W3037335012 @default.
• W4288712745 cites W3092221168 @default.
• W4288712745 cites W4211223133 @default.
• W4288712745 doi "https://doi.org/10.1021/jasms.2c00113" @default.
• W4288712745 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/35905433" @default.
• W4288712745 hasPublicationYear "2022" @default.
• W4288712745 type Work @default.
• W4288712745 citedByCount "0" @default.
• W4288712745 crossrefType "journal-article" @default.
• W4288712745 hasAuthorship W4288712745A5011972457 @default.
• W4288712745 hasAuthorship W4288712745A5019770299 @default.
• W4288712745 hasAuthorship W4288712745A5033119802 @default.
• W4288712745 hasAuthorship W4288712745A5036433151 @default.
• W4288712745 hasAuthorship W4288712745A5069278408 @default.
• W4288712745 hasAuthorship W4288712745A5073114604 @default.
• W4288712745 hasAuthorship W4288712745A5076661275 @default.
• W4288712745 hasConcept C111368507 @default.
• W4288712745 hasConcept C113196181 @default.
• W4288712745 hasConcept C127313418 @default.
• W4288712745 hasConcept C134018914 @default.
• W4288712745 hasConcept C145148216 @default.
• W4288712745 hasConcept C147789679 @default.
• W4288712745 hasConcept C148065180 @default.
• W4288712745 hasConcept C162356407 @default.
• W4288712745 hasConcept C17525397 @default.
• W4288712745 hasConcept C178790620 @default.
• W4288712745 hasConcept C185592680 @default.
• W4288712745 hasConcept C198291218 @default.
• W4288712745 hasConcept C200239111 @default.
• W4288712745 hasConcept C25366896 @default.
• W4288712745 hasConcept C2776923573 @default.
• W4288712745 hasConcept C2777379467 @default.
• W4288712745 hasConcept C2778541603 @default.
• W4288712745 hasConcept C43617362 @default.
• W4288712745 hasConcept C51884965 @default.
• W4288712745 hasConcept C518881349 @default.
• W4288712745 hasConcept C68801617 @default.
• W4288712745 hasConcept C71924100 @default.
• W4288712745 hasConceptScore W4288712745C111368507 @default.
• W4288712745 hasConceptScore W4288712745C113196181 @default.
• W4288712745 hasConceptScore W4288712745C127313418 @default.
• W4288712745 hasConceptScore W4288712745C134018914 @default.
• W4288712745 hasConceptScore W4288712745C145148216 @default.
• W4288712745 hasConceptScore W4288712745C147789679 @default.
• W4288712745 hasConceptScore W4288712745C148065180 @default.
• W4288712745 hasConceptScore W4288712745C162356407 @default.
• W4288712745 hasConceptScore W4288712745C17525397 @default.
• W4288712745 hasConceptScore W4288712745C178790620 @default.
• W4288712745 hasConceptScore W4288712745C185592680 @default.
• W4288712745 hasConceptScore W4288712745C198291218 @default.
• W4288712745 hasConceptScore W4288712745C200239111 @default.
• W4288712745 hasConceptScore W4288712745C25366896 @default.
• W4288712745 hasConceptScore W4288712745C2776923573 @default.
• W4288712745 hasConceptScore W4288712745C2777379467 @default.
• W4288712745 hasConceptScore W4288712745C2778541603 @default.
• W4288712745 hasConceptScore W4288712745C43617362 @default.

• next