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- W4289076803 abstract "Negative thermal expansion (NTE) in Bi0.5+xNa0.5−xVO3 is investigated. The parent compound, Bi0.5Na0.5VO3, is a lead-free polar perovskite oxide with a tetragonal distortion comparable to that of ferroelectric PbTiO3 owing to the ordering of dxy orbital of V4+ with d1 electronic configuration. The c/a ratio was decreased by electron doping to V4+ through increasing Bi3+/Na+ ratio and transition to a non-polar cubic phase on heating accompanied by NTE with a large volume shrinkage of −2.28 % was enabled. It is found that the Bi0.5Na0.5VO3 derivatives exhibit NTE when the c/a ratio is smaller than the critical value of ∼1.06." @default.
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- W4289076803 date "2022-08-01" @default.
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- W4289076803 title "Negative thermal expansion in PbTiO<sub>3</sub>-type perovskites oxide Bi<sub>0.5+</sub><i><sub>x</sub></i>Na<sub>0.5−</sub><i><sub>x</sub></i>VO<sub>3</sub>" @default.
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- W4289076803 doi "https://doi.org/10.2109/jcersj2.22059" @default.
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