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• W4289109743 abstract "Abstract The universal limit on the pH conditions is disturbing peroxymonosulfate (PMS)‐triggered high‐valent iron‐oxo systems in environmental applications. Here, we propose for the first time the construction of a neutral microenvironment on the surface of Zn−Fe layered double hydroxide (ZnFe‐LDH) by using the amphoteric properties of zinc hydroxide, which continuously generates ≡Fe IV =O over a wide pH range of 3.0–11.0 in activating PMS. The ≡Zn(OH) 2 moiety offers a neutral microenvironment at the phase interface, which mitigates the self‐decomposition of ≡Fe IV =O by protons and the hydrolysis reaction of iron by hydroxyl groups, which is supported by the Mossbauer spectra, density functional theory calculations and designed experiments. Consequently, ZnFe‐LDH/PMS can satisfy the stability in long‐term experiments, selectivity under conditions with high salinity or natural organic matter and efficient treatment of actual wastewater." @default.
• W4289109743 created "2022-08-01" @default.
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• W4289109743 date "2022-08-17" @default.
• W4289109743 modified "2023-10-18" @default.
• W4289109743 title "Generating High‐valent Iron‐oxo ≡Fe^IV=O Complexes in Neutral Microenvironments through Peroxymonosulfate Activation by Zn−Fe Layered Double Hydroxides" @default.
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• W4289109743 doi "https://doi.org/10.1002/ange.202209542" @default.
• W4289109743 hasPublicationYear "2022" @default.
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