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- W4289260707 abstract "The oxygen reduction reaction (ORR) on the low- and high-index planes of Pt modified with a protonic ionic liquid ([7-methyl-1,5,7-triazabicyclo(4.4.0)dec-5-ene][bis(pentafluoroethylsulfonyl)imide], referred to here as [MTBD][beti]) was studied in 0.1 M perchloric acid solution. The specific activity of the ORR on Pt(1 1 1) modified with [MTBD][beti] was 3.1 times higher than that on unmodified Pt(1 1 1), while the ORR was deactivated on modified Pt(1 0 0). [MTBD][beti] slightly enhanced the ORR activity of the Pt n(1 1 1)–(1 1 1) planes (where n = 2–9). These results show that a larger (1 1 1) terrace is essential for a marked increase in the ORR activity on Pt electrodes modified with [MTBD][beti]. Although the ratio of the increase in the activity of n(1 1 1)–(1 1 1) was lower than that of Pt(1 1 1), Pt(3 3 1) = 3(1 1 1)–(1 1 1) showed the highest ORR activity after [MTBD][beti] modification. The effects of MTBD and beti were also studied separately. MTBD provided the main contribution to the increase in ORR activity, giving the highest activity at a concentration of 2.0–3.5 × 10–5 M, whereas beti affected the ORR activity only slightly." @default.
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- W4289260707 date "2022-07-01" @default.
- W4289260707 modified "2023-09-23" @default.
- W4289260707 title "Oxygen reduction reaction on platinum single-crystal electrodes modified with protonic ionic liquid" @default.
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- W4289260707 doi "https://doi.org/10.1016/j.elecom.2022.107337" @default.
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