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• W4289308561 startingPage "2200337" @default.
• W4289308561 abstract "The structure and components of solid electrolyte interphase (SEI) is crucial to direct the growth of lithium particles. However, it is hard to have control over them. Herein, an SEI that shares the properties of Li2CO3-rich and LiF-rich types is realized by using different fluorine phenylphospines, and constructing a Li2CO3/LiF-rich heterostructured SEI by using tris(4-fluorophenyl)phosphine (TFPP) as the electrolyte additive. The well-balanced SEI formed in TFPP-containing electrolyte has the fast Li+ transport kinetics of Li2CO3, good electron insulator capability of LiF, and strong affinity toward Li+. It can effectively guarantee fast, uniform Li+ flux through the SEI while preventing electrons from the Li anode entering into SEI, and thus realizes uniform and dense Li deposition at the SEI/Li interface. As expected, the Li anode with TFPP-containing electrolyte achieves a stable Li plating/stripping over 400 h at 1mA cm−2 while the full cell with a high-voltage LiNi0.6Co0.2Mn0.2O2 cathode also enables long-term stability with a capacity retention (87.8% after 200 cycles) at 0.1 A g−1 and excellent rate performance." @default.
• W4289308561 created "2022-08-02" @default.
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• W4289308561 date "2022-03-23" @default.
• W4289308561 modified "2023-10-11" @default.
• W4289308561 title "Li ₂ CO ₃ /LiF‐Rich Heterostructured Solid Electrolyte Interphase with Superior Lithiophilic and Li ⁺ ‐Transferred Characteristics via Adjusting Electrolyte Additives" @default.
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• W4289308561 doi "https://doi.org/10.1002/aenm.202200337" @default.
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