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• W4289443604 abstract "Electrochemical production of hydrogen peroxide (H2 O2 ) from O2 on single-atom catalysts has attracted great attention, yet the quest for robust catalysts is driven by achieving >90 % Faradaic efficiency (FE) under industrial-relevant current densities (>100 mA cm-2 ). Herein we synthesize a catalyst that contains single nickel site coordinated by four nitrogen and two oxygen atoms (i.e., N4 Ni1 O2 ) via involving carboxyl functionalized multiwall carbon nanotubes as a substrate to provide extra O coordination to the regular NiN4 site. It has a cathodic energy efficiency of approximately 82 % and a H2 O2 FE of around 96 % at 200 mA cm-2 current density, outperforming the reported single-atom catalysts for H2 O2 electrosynthesis." @default.
• W4289443604 created "2022-08-02" @default.
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• W4289443604 date "2022-08-16" @default.
• W4289443604 modified "2023-10-17" @default.
• W4289443604 title "Super‐Coordinated Nickel N₄Ni₁O₂ Site Single‐Atom Catalyst for Selective H₂O₂ Electrosynthesis at High Current Densities" @default.
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• W4289443604 doi "https://doi.org/10.1002/anie.202206544" @default.
• W4289443604 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/35916327" @default.
• W4289443604 hasPublicationYear "2022" @default.
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