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• W4289711596 abstract "An asymmetric para-C(sp2 )-H bond functionalization of alkyl benzene derivatives was successfully developed via cooperative catalysis of gold and chiral phosphoric acid (CPA), leading to synthetically useful chiral 1,1-diaryl motifs. Chiral phosphoric acid, ligand, and molecular sieves were found to be crucial for enantioselectivity control of this transformation. The salient features of this protocol include mild conditions, high efficiency, commercially available starting materials, highly chemo- and site- as well as enantioselective aromatic C-H functionalization, broad substrate scope, and extensive applications of the chiral products. The mechanistic studies suggested that two CPAs might be involved in chiral induction." @default.
• W4289711596 created "2022-08-04" @default.
• W4289711596 creator A5040585691 @default.
• W4289711596 creator A5049264813 @default.
• W4289711596 creator A5049900943 @default.
• W4289711596 creator A5071833362 @default.
• W4289711596 creator A5080524490 @default.
• W4289711596 creator A5086503621 @default.
• W4289711596 date "2022-08-24" @default.
• W4289711596 modified "2023-10-17" @default.
• W4289711596 title "Enantioselective <i>para</i> ‐C(sp ² )−H Functionalization of Alkyl Benzene Derivatives via Cooperative Catalysis of Gold/Chiral Brønsted Acid**" @default.
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