Matches in SemOpenAlex for { <https://semopenalex.org/work/W4289885514> ?p ?o ?g. }
- W4289885514 endingPage "546" @default.
- W4289885514 startingPage "535" @default.
- W4289885514 abstract "Plasma-surface coupling has emerged as a promising approach to perform chemical transformations under mild conditions that are otherwise difficult or impossible thermally. However, a few examples of inexpensive and accessible in situ/operando techniques exist for observing plasma-solid interactions, which has prevented a thorough understanding of underlying surface mechanisms. Here, we provide a simple and adaptable design for a dielectric barrier discharge (DBD) plasma cell capable of interfacing with Fourier transform infrared spectroscopy (FTIR), optical emission spectroscopy (OES), and mass spectrometry (MS) to simultaneously characterize the surface, the plasma phase, and the gas phase, respectively. The system was demonstrated using two example applications: (1) plasma oxidation of primary amine functionalized SBA-15 and (2) catalytic low temperature nitrogen oxidation. The results from application (1) provided direct evidence of a 1% O2/He plasma interacting with the aminosilica surface by selective oxidation of the amino groups to nitro groups without altering the alkyl tether. Application (2) was used to detect the evolution of NOX species bound to both platinum and silica surfaces under plasma stimulation. Together, the experimental results showcase the breadth of possible applications for this device and confirm its potential as an essential tool for conducting research on plasma-surface coupling." @default.
- W4289885514 created "2022-08-05" @default.
- W4289885514 creator A5029631906 @default.
- W4289885514 creator A5043778579 @default.
- W4289885514 date "2022-08-05" @default.
- W4289885514 modified "2023-10-01" @default.
- W4289885514 title "<b>Interrogation of the Plasma-Catalyst Interface via In Situ/Operando Transmission Infrared Spectroscopy</b>" @default.
- W4289885514 cites W1644173725 @default.
- W4289885514 cites W1708754953 @default.
- W4289885514 cites W1876337511 @default.
- W4289885514 cites W194148622 @default.
- W4289885514 cites W1965026276 @default.
- W4289885514 cites W1966320365 @default.
- W4289885514 cites W1967743582 @default.
- W4289885514 cites W1979578011 @default.
- W4289885514 cites W1980953390 @default.
- W4289885514 cites W1983059445 @default.
- W4289885514 cites W1986078565 @default.
- W4289885514 cites W1991427575 @default.
- W4289885514 cites W1995041236 @default.
- W4289885514 cites W1997283548 @default.
- W4289885514 cites W1998871781 @default.
- W4289885514 cites W2000433958 @default.
- W4289885514 cites W2001825008 @default.
- W4289885514 cites W2005258639 @default.
- W4289885514 cites W2005271134 @default.
- W4289885514 cites W2013130926 @default.
- W4289885514 cites W2015020080 @default.
- W4289885514 cites W2016844892 @default.
- W4289885514 cites W2017633570 @default.
- W4289885514 cites W2027792673 @default.
- W4289885514 cites W2037219273 @default.
- W4289885514 cites W2041755910 @default.
- W4289885514 cites W2052139646 @default.
- W4289885514 cites W2058199646 @default.
- W4289885514 cites W2067320964 @default.
- W4289885514 cites W2070286510 @default.
- W4289885514 cites W2074525088 @default.
- W4289885514 cites W2075276936 @default.
- W4289885514 cites W2076828327 @default.
- W4289885514 cites W2080170858 @default.
- W4289885514 cites W2081527912 @default.
- W4289885514 cites W2083905016 @default.
- W4289885514 cites W2086722940 @default.
- W4289885514 cites W2087872498 @default.
- W4289885514 cites W2128417034 @default.
- W4289885514 cites W2129000212 @default.
- W4289885514 cites W2133932638 @default.
- W4289885514 cites W2149248689 @default.
- W4289885514 cites W2237787486 @default.
- W4289885514 cites W2247746448 @default.
- W4289885514 cites W2275798544 @default.
- W4289885514 cites W2316374104 @default.
- W4289885514 cites W2318775926 @default.
- W4289885514 cites W2345701936 @default.
- W4289885514 cites W2349312798 @default.
- W4289885514 cites W2395841795 @default.
- W4289885514 cites W2488757668 @default.
- W4289885514 cites W2489802352 @default.
- W4289885514 cites W2496302860 @default.
- W4289885514 cites W2529665182 @default.
- W4289885514 cites W2548253516 @default.
- W4289885514 cites W2592943737 @default.
- W4289885514 cites W2610137023 @default.
- W4289885514 cites W2626197741 @default.
- W4289885514 cites W2734710772 @default.
- W4289885514 cites W2743465261 @default.
- W4289885514 cites W2746397488 @default.
- W4289885514 cites W2759696274 @default.
- W4289885514 cites W2785311975 @default.
- W4289885514 cites W2803852160 @default.
- W4289885514 cites W2904788502 @default.
- W4289885514 cites W2910984700 @default.
- W4289885514 cites W2911797404 @default.
- W4289885514 cites W2922139270 @default.
- W4289885514 cites W2922150777 @default.
- W4289885514 cites W2929739531 @default.
- W4289885514 cites W2933838996 @default.
- W4289885514 cites W2939640222 @default.
- W4289885514 cites W2967451225 @default.
- W4289885514 cites W3005305727 @default.
- W4289885514 cites W3011042875 @default.
- W4289885514 cites W3013335807 @default.
- W4289885514 cites W3023530634 @default.
- W4289885514 cites W3028242135 @default.
- W4289885514 cites W3069753755 @default.
- W4289885514 cites W3108866557 @default.
- W4289885514 cites W3118190597 @default.
- W4289885514 cites W3118434330 @default.
- W4289885514 cites W3120457537 @default.
- W4289885514 cites W3133822769 @default.
- W4289885514 cites W3159787008 @default.
- W4289885514 cites W3168643605 @default.
- W4289885514 cites W3195376005 @default.
- W4289885514 cites W3214343630 @default.
- W4289885514 cites W3214531017 @default.
- W4289885514 cites W35371265 @default.
- W4289885514 cites W4200493475 @default.