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- W4290802445 abstract "Fast electron impact was used to study the generalized oscillator strengths of the inner-shell excitations in atoms and molecules previously. In this work, a nonresonant inelastic x-ray scattering technique is extended to determine the generalized oscillator strengths of $(1{ensuremath{sigma}}_{g}ensuremath{rightarrow}1{ensuremath{pi}}_{g})+(1{ensuremath{sigma}}_{u}ensuremath{rightarrow}1{ensuremath{pi}}_{g})$ inner-shell excitations of molecular nitrogen in the squared momentum transfer range of 0.86 to 14.40 a.u. at a photon energy of about 10 keV and an energy resolution of about 1.3 eV. The present generalized oscillator strength strictly follows the first Born approximation and thus provides a rigorous test to the previously calculated results and the experimental ones measured by the electron energy loss spectroscopy. The presently extrapolated optical oscillator strength at zero momentum transfer is in accord with most experimental results and the theoretical data with the correlation effect considered carefully. This work indicates that the nonresonant inelastic x-ray scattering technique is a powerful tool to study the core excitation mechanism in atoms and molecules." @default.
- W4290802445 created "2022-08-12" @default.
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- W4290802445 date "2022-08-11" @default.
- W4290802445 modified "2023-10-17" @default.
- W4290802445 title "Generalized oscillator strength of the core-excited states of molecular nitrogen studied by nonresonant inelastic x-ray scattering" @default.
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- W4290802445 doi "https://doi.org/10.1103/physreva.106.022806" @default.
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