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- W4290852303 abstract "Facile conversion of petrochemical feedstocks into valuable amine molecules remains a long-standing challenge in organic chemistry. Here, we report a modular and practical alkene 1,1-carboamination technology that relies on sequential azo-ene reactions and attendant base-promoted N-N bond cleavage of azo-ene adducts with Grignard reagents. By employing allylic urazoles as imine surrogates, this method bypasses the conventional retrosynthetic logic of imine synthesis, thereby allowing for rapid access to diverse α-branched allylic amine derivatives." @default.
- W4290852303 created "2022-08-12" @default.
- W4290852303 creator A5076156449 @default.
- W4290852303 date "2022-08-12" @default.
- W4290852303 modified "2023-10-16" @default.
- W4290852303 title "1,1-Carboamination of Terminal Alkenes via a Reaction of Azo-Ene Adducts with Grignard Reagents" @default.
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- W4290852303 doi "https://doi.org/10.1021/acs.orglett.2c02585" @default.
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