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- W4291008681 abstract "Regulating local electron density by introducing single-atom is an effective strategy to improve the activity of heterogeneous photo-Fenton processes. Here N, P coordinated Fe and Ni single-atom catalysts on carbon nitrides (CN-FeNi-P) were prepared to activate H2O2 for contaminant mineralization under visible light irradiation. The as-prepared CN-FeNi-P presented a higher moxifloxacin degradation activity in photo-Fenton system, which was up to 3.7 times that of pristine CN, meanwhile, its TOC removal reached to 95.9 % in 60 min. Based on density functional theory calculations, the Ni single-atoms serve as the optimal reactive sites to produce •OH. The strong interaction between Fe and Ni single-atoms by P-bridging and the modulated local electron structure after introducing P into coordination environment can lower •OH formation energy. This study provides new doping strategies to design single-atom catalysts and expands the family of the Fenton-like system for advanced oxidation technologies." @default.
- W4291008681 created "2022-08-13" @default.
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- W4291008681 date "2022-10-01" @default.
- W4291008681 modified "2023-10-11" @default.
- W4291008681 title "Regulating electron distribution of Fe/Ni-N4P2 single sites for efficient photo-Fenton process" @default.
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- W4291008681 doi "https://doi.org/10.1016/j.jhazmat.2022.129724" @default.
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