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• W4291221701 endingPage "129940" @default.
• W4291221701 startingPage "129940" @default.
• W4291221701 abstract "Bi-based semiconductors have been regarded to be an ideal platform in photocatalytic CO2 reduction to fuels. However, the insufficient charge transfer efficiency greatly restricts their practical application. Herein, we fabricated 1D/2D hierarchical heterostructures by the hybridization of Bi4O5Br2 and rod-like MOF-derived MoS2 anchored in nitrogen-doped porous carbon (NPC-MoS2) using Mo-MOF as a precursor followed by sulfidation and typical solvothermal process. Compared to pristine Bi4O5Br2 nanosheet and NPC-MoS2 nanorod, the 5 wt% NPC-MoS2@Bi4O5Br2 p-n heterojunction exhibits distinctly enhanced photocatalytic activity under light illumination due to the increased light absorption capability and more effective charge transfer efficiency. X-ray photoelectron spectroscopy and photoelectrochemical analysis imply that a built-in electric field on interfaces is created to form p-n heterojunctions which drive the photoinduced electrons transferred from NPC-MoS2 to Bi4O5Br2. Finally, the type-II charge transfer mechanism is proposed which promotes separation of the charges and provides suitable conduction band to reduce CO2 much efficiently. In a word, this work provides a new insight into the establishment of hierarchical p-n heterostructures for photocatalysis." @default.
• W4291221701 created "2022-08-13" @default.
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• W4291221701 date "2022-11-01" @default.
• W4291221701 modified "2023-10-15" @default.
• W4291221701 title "Fabrication of Bi4O5Br2-decorated rod-like MOF-derived MoS2 hierarchical heterostructures for boosting photocatalytic CO2 reduction" @default.
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• W4291221701 doi "https://doi.org/10.1016/j.colsurfa.2022.129940" @default.
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