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- W4291638262 abstract "In aqueous electrolyte, the hydration of solvated zinc ions and the unstable deposition interface exacerbate the accumulation of Zn dendrites and the generation of by-products, making it difficult to achieve highly reversible and long-life Zn-ion batteries (ZIBs). Herein, a high-modulus agarose gel electrolyte (AGE) with greatly suppressed H2O molecule mobility, is designed to overcome the above challenges. The ample hydroxyl (-OH) functional groups on the double helix chain of the AGE can capture and anchor H2O molecules via hydrogen bonding, thus fundamentally regulating the coordination environment of Zn2+ and enhancing the stability of deposition interface. Moreover, the -OH functional groups can also effectively immobilize sulfate ions and largely confine their free diffusion, thereby greatly inhibiting the formation of zinc hydroxysulfate by-product. As such, the dendrite issue and side reactions can be significantly mitigated using our designed AGEs, holding great promise for ZIBs with extended cycling durability and high safety." @default.
- W4291638262 created "2022-08-15" @default.
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- W4291638262 date "2022-10-01" @default.
- W4291638262 modified "2023-10-18" @default.
- W4291638262 title "Stable Zn anodes enabled by high-modulus agarose gel electrolyte with confined water molecule mobility" @default.
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- W4291638262 doi "https://doi.org/10.1016/j.electacta.2022.140985" @default.
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