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• W4291779969 abstract "The synthesis and characterisation of a library of acyclic antimony(III) and bismuth(III) triaryl pnictogen bonding (PnB) receptor systems are reported. In the first-generation receptor series, quantitative 1H NMR chloride titration experiments in THF solvent media reveal halide anion binding potency is intimately correlated with both the electronic-withdrawing nature of the aryl- substituent and the polarisability of the PnB donor. Further extensive anion binding investigations with the most potent Sb- and Bi-based PnB receptors: 1⋅Sb2CF3 and 1⋅Bi2CF3, reveal novel selectivity profiles, both displaying Cl− selectivity relative to the heavier halides and, impressively, to a range of highly basic oxoanions. The synthesis and preliminary chloride anion binding studies of a series of novel tripodal tris-proto-triazole triaryl Sb(III) and Bi(III) mixed PnB-HB receptor systems are also described. Whereas parent triphenyl Sb(III) and Bi(III) compounds are incapable of binding Cl− in THF solvent media, the PnB-triazole HB host systems exhibit notable halide affinity." @default.
• W4291779969 created "2022-08-16" @default.
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• W4291779969 date "2022-10-11" @default.
• W4291779969 modified "2023-09-30" @default.
• W4291779969 title "Anion Recognition with Antimony(III) and Bismuth(III) Triaryl‐Based Pnictogen Bonding Receptors" @default.
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• W4291779969 doi "https://doi.org/10.1002/chem.202201838" @default.
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