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- W4292014254 abstract "Abstract Porous liquid is a unique liquid medium that combines permanent porosity of porous solid with the fluidity of liquid, and this special characteristic makes it potential in various applications. Here we report the first photoresponsive porous ionic liquid (PPIL) by solubilizing photoresponsive metal-organic polyhedron (PMOP, constructed from dicopper and azobenzene-containing carboxylate) in polyethylene-glycol-functionalized bulky ionic liquid (IL). Owing to favorable ion interactions, bulky IL molecules encircle outside PMOP cages, and the inter cavities are maintained. The azobenzene moieties can be isomerized freely in the obtained PPILs to expose and shelter active sites upon visible and UV light irradiations. Hence, the adsorption capacity of PPILs is controllable by light irradiation, and the change in CO 2 uptake is up to 30% which is different from neat IL with negligible change. This study might inspire the development of new adsorption process regulated by light instead of conventional pressure and temperature swing adsorption technologies." @default.
- W4292014254 created "2022-08-17" @default.
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- W4292014254 date "2022-08-16" @default.
- W4292014254 modified "2023-09-26" @default.
- W4292014254 title "Porous Liquids Responsive to Light" @default.
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- W4292014254 doi "https://doi.org/10.21203/rs.3.rs-1430877/v1" @default.
- W4292014254 hasPublicationYear "2022" @default.
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