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• W4292396013 endingPage "141073" @default.
• W4292396013 startingPage "141073" @default.
• W4292396013 abstract "Lithium metal batteries (LMBs) with ultra-high theoretical energy density are a prospective candidate to replace current lithium-ion batteries (LIBs). However, there are still two non-negligible problems of lithium dendrites and the volume expansion effect of LMBs. In this study, reduced graphene oxide (rGO)/Li-Al-LDH composite nanosheets were firstly prepared via a hydrothermal method and then vacuum filtered onto commercial polypropylene (PP) separator. This kind of rGO/Li-Al-LDH nanosheets layer is expected to improve the wettability of liquid electrolytes and thermal stability. Furthermore, rich- Li-Al LDH can promote more ionic carriers and channels, which exhibits higher-efficiency lithium-ion transport properties. Meanwhile, rGO with a graphitic-like structure is able to disperse the concentration of electrons at the sharp point when lithium dendrites arise. As a result, the discharge capacity of the Li||LiFePO4 cells based on the rGO/[email protected] separator is still 1.852 mAh after 250 cycles and the capacity decay rate is just 4.24%. It is demonstrated that a feasible and effective strategy for the modified separator can enhance the electrochemical performance of LMBs." @default.
• W4292396013 created "2022-08-20" @default.
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• W4292396013 date "2022-10-01" @default.
• W4292396013 modified "2023-10-08" @default.
• W4292396013 title "rGO/Li-Al-LDH composite nanosheets modified commercial polypropylene (PP) separator to suppress lithium dendrites for lithium metal battery" @default.
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• W4292396013 doi "https://doi.org/10.1016/j.electacta.2022.141073" @default.
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