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- W4292595315 abstract "Plasmonic photoelectrochemical (PEC) water splitting has excited immense interest, as it can overcome the intrinsic limitations of semiconductors, in terms of light absorption, by the localized-surface plasmon resonances effect. Here, to get insight into the role of plasmonic hot carriers in plasmonic water splitting, a rational design of an antenna–reactor type Pt/Ag/TiO 2 metal–semiconductor Schottky nanodiode was fabricated and used as a photoanode. Using the designed PEC cell system combined with the Pt/Ag/TiO 2 nanodiode, we show that the plasmonic hot carriers excited from Ag were utilized for the oxygen (O 2 ) evolution reaction and, consequently, had a decisive role in the enhancement of the photocatalytic efficiency. These results were supported by finite-difference time-domain simulations, and the faradaic efficiency was measured by the amount of actual gas produced. Therefore, this study provides a deep understanding of the dynamics and mechanisms of plasmonic hot carriers in plasmonic-assisted PEC water splitting." @default.
- W4292595315 created "2022-08-22" @default.
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- W4292595315 date "2022-08-28" @default.
- W4292595315 modified "2023-10-16" @default.
- W4292595315 title "Plasmonic hot carrier-driven photoelectrochemical water splitting on antenna–reactor Pt/Ag/TiO<sub>2</sub> Schottky nanodiodes" @default.
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- W4292595315 doi "https://doi.org/10.1063/5.0097713" @default.
- W4292595315 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/36050032" @default.
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