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- W4292622280 abstract "Two-dimensional (2D) interlayer confined channels of graphene oxide (GO) membrane and their potential for ultrafast water molecules transport behavior have drawn substantial interest for advanced water-related membrane separation process. However, the water transfer pathways along the edge-to-edge slits to interlayer channels of adjacent GO nanosheets are still very tortuous, leading to low-efficiency water permeation. Herein, we designed and prepared hollow zeolitic imidazolate framework-8 nanocrystals with enhanced hydrophilic surface ([email protected]), and then they were incorporated into GO membrane to introduce more nanofluidic channels. More importantly, the enhanced-surface hydrophilicity could well capture water molecules and make them diffuse along the porous multi-pathways of [email protected] and interlayer channels of GO, further reducing mass transfer resistance and improving water transfer efficiency under highly-water chemical potential driving force in membrane microregion. As-prepared [email protected]/GO membrane on polyethersulfone (PES) substrate with optimum structure showed the pure water flux as high as 32.11 kg m−2 h−1 at 323 K, and meanwhile exhibited superior pervaporation dehydration performance of butanol/water mixture with total flux of 5.32 kg m−2 h−1 and separation factor of 3567 at 343 K, respectively. This work strengthens the understanding of high-efficiency water transport along multi-dimensional heterogenous channels in advanced 2D separation membranes." @default.
- W4292622280 created "2022-08-22" @default.
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- W4292622280 date "2022-11-01" @default.
- W4292622280 modified "2023-10-17" @default.
- W4292622280 title "Two-dimensional heterogenous channels incorporated by enhanced-surface hydrophilic hollow ZIF-8 nanocrystals for ultrafast water permeation" @default.
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- W4292622280 doi "https://doi.org/10.1016/j.memsci.2022.120943" @default.
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