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• W4292819919 endingPage "125493" @default.
• W4292819919 startingPage "125493" @default.
• W4292819919 abstract "A series of Al-SBA-15 were synthesized with three Al introduction methods and different Si/Al molar ratios. The introduction methods included the direct synthesis (DS), post-synthesis grafting (PG) and impregnation synthesis (IM) method. The Si/Al molar ratios of Al-SBA-15 materials were 20, 10 and 5 respectively. The corresponding NiMoS catalysts were performed by hydrodesulfurization (HDS) recations of dibenzothiophene (DBT) to analyze reaction behavior. The characterization results of N2-physisorption, X-ray diffraction and 27Al NMR presented that the Al introduction method has a direct effect on the physical and chemical properties of Al-SBA-15. PG method could introduce most of Al atoms into the framework of parent- material, which was opposed to the IM method. The DS method could better maintain the pore structure advantages of the Al-SBA-15. The PG-NiMo catalyst had the strongest metal-support interaction, and the NiMoS slabs presented the lowest average stacking number over this catalyst. The reaction results showed that DS-NiMo catalyst obtained the highest HDS activity, and PG-NiMo catalyst presented the highest HDS hydrogenolysis selectivity of DBT. It is speculated that the frame-work Al has strong metal interaction with metal oxide precursor, and the morphology of NiMoS Phase has important effect on the selectivity of DBT HDS." @default.
• W4292819919 created "2022-08-24" @default.
• W4292819919 creator A5044960363 @default.
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• W4292819919 date "2022-12-01" @default.
• W4292819919 modified "2023-09-28" @default.
• W4292819919 title "Effects of Al introduction methods for Al-SBA-15 on NiMoS active phase morphology and hydrodesulfurization reaction selectivities" @default.
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• W4292819919 doi "https://doi.org/10.1016/j.fuel.2022.125493" @default.
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