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- W4293049258 abstract "Difluoroenol silyl ethers are a unique class of enol silyl ethers that are widely used as a powerful difluoroalkylating reagent to incorporate difluoromethylene groups into organic molecules. In this context, we revealed a fluorine effect that the difluoroenol silyl ethers exhibit the oxygen nucleophilicity in lieu of traditional α-carbon nucleophilicity toward the aromatic iodonium/sulfonium species, thus allowing us to develop difluoroalkylative [3,3]-rearrangement of aryl iodanes and aryl sulfoxides and the difluoroalkylative dearomatization of aryl sulfoxides. In this article, we summarize these works and illustrate the logic of our design." @default.
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- W4293049258 date "2022-08-25" @default.
- W4293049258 modified "2023-09-28" @default.
- W4293049258 title "Aromatic iodonium/sulfonium rearrangement using difluoroenol silyl ethers" @default.
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- W4293049258 doi "https://doi.org/10.1080/10426507.2022.2113977" @default.
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