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- W4293216066 abstract "Metastable iron oxide (β-Fe2O3) has attracted wide attention in photoelectrochemical water splitting as a result of its ideal light absorption capacity and theoretical saturation photocurrent. However, the poor crystallinity and high concentration of defects of β-Fe2O3 prepared by the traditional method resulted in a high onset potential in photoelectrochemical water splitting. This work proved that γ-Fe2O3 can be converted into β-Fe2O3 under heating, which exploits a new synthetic route for β-Fe2O3. β-Fe2O3 obtained by this phase transformation method has a smaller particle size and better crystallinity, resulting in a significant reduction in defects. The β-Fe2O3 photoanode exhibits an onset potential below 0.8 VRHE, which is the lowest data thus far. This discovery breaks through the limited synthesis methods of β-Fe2O3, thereby reducing the obstacles of preparing β-Fe2O3 photoelectrodes." @default.
- W4293216066 created "2022-08-27" @default.
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- W4293216066 date "2022-08-24" @default.
- W4293216066 modified "2023-10-16" @default.
- W4293216066 title "Onset Potential Shift of Water Oxidation in the Metastable Phase Transformation Process of β-Fe<sub>2</sub>O<sub>3</sub>" @default.
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- W4293216066 doi "https://doi.org/10.1021/acs.energyfuels.2c01812" @default.
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