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• W4293232245 abstract "A series of Pd1-x Fe x alloy epitaxial films (x = 0, 0.038, 0.062, and 0.080), a material promising for superconducting spintronics, was prepared and studied with ultrafast optical and magneto-optical laser spectroscopy in a wide temperature range of 4-300 K. It was found that the transition to the ferromagnetic state causes a qualitative change of both the reflectivity and the magneto-optical Kerr effect transients. A nanoscale magnetic inhomogeneity of the ferromagnet/paramagnet type inherent in the palladium-rich Pd1-x Fe x alloys reveals itself through the occurrence of a relatively slow, 10-25 ps, photoinduced demagnetization component following a subpicosecond one; the former vanishes at low temperatures only in the x = 0.080 sample. We argue that the 10 ps timescale demagnetization originates most probably from the diffusive transport of d electrons under the condition of nanoscale magnetic inhomogeneities. The low-temperature fraction of the residual paramagnetic phase can be deduced from the magnitude of the slow reflectivity relaxation component. It is estimated as ≈30% for x = 0.038 and ≈15% for x = 0.062 films. The minimal iron content ensuring the magnetic homogeneity of the ferromagnetic state in the Pd1-x Fe x alloy at low temperatures is about 7-8 atom %." @default.
• W4293232245 created "2022-08-27" @default.
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• W4293232245 date "2022-08-25" @default.
• W4293232245 modified "2023-09-28" @default.
• W4293232245 title "Ultrafast signatures of magnetic inhomogeneity in Pd₁₋<i>_x</i>Fe<i>_x</i> (<i>x</i> ≤ 0.08) epitaxial thin films" @default.
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• W4293232245 doi "https://doi.org/10.3762/bjnano.13.74" @default.
• W4293232245 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/36105688" @default.
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