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- W4293240619 abstract "Cobalt nitrides with a high ratio of cobalt–cobalt interaction have been extensively explored as electrocatalysts for hydrogen evolution reaction (HER) catalysis. However, the tilted orbital orientation and limited empty d ‐orbitals above the Fermi level ( E F ) result in unfavorable water adsorption/activation. Herein, facile interfacial engineering by in situ growing of MoN particles on Co 4 N nanowire arrays to explore the interfacial synergistic mechanism for boosting HER catalysis is developed. The overpotential of the prepared MoN–Co 4 N at 10 mA cm −2 is only 45.1 mV, which is substantially better than the pristine Co 4 N (207 mV). According to density functional theory (DFT) calculations, MoN with vertical orbital orientation and more empty d ‐orbitals above E F contributes to water adsorption and activation, while the Co 4 N surface is responsible for the adsorption/desorption of the intermediate H. Understanding the synergistic effects of each catalytic component at the atomic levels offers valuable insights for rational design of efficient HER catalysts and beyond." @default.
- W4293240619 created "2022-08-27" @default.
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- W4293240619 date "2022-04-28" @default.
- W4293240619 modified "2023-10-15" @default.
- W4293240619 title "Constructing Complementary Catalytic Components on Co<sub>4</sub>N Nanowires to Achieve Efficient Hydrogen Evolution Catalysis" @default.
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- W4293240619 doi "https://doi.org/10.1002/aesr.202100219" @default.
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