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- W4293385909 abstract "A series of Ni-xCe/CNTs were synthesized by incipient wetness impregnation method and characterized by XRD, XPS, and H 2 -TPR. Their catalytic performances were systematically evaluated in hydrothermal liquefaction of Tetra Pak. The effects of Ni:Ce ratio (10:0–10:7) in the bio-oil yield, boiling point, elemental composition, higher heating value (HHV) and chemical components of the bio-oil were investigated, and the solid residue and the used catalysts were also analyzed by TG, FT-IR and XRD, SEM, respectively. Maximum bio-oil yield of 20.75 wt% was obtained at Ni:Ce of 10:5. The minimum crystallite size of CeO 2 and the highest Ce 3+ concentration, respecting the highest oxygen vacancies was obtained for Ni–5Ce/CNTs by XRD, and the lowest reduction temperature was also found for Ni–5Ce/CNTs in H 2 -TPR analysis, indicating the good reducibility. The CeO 2 became to accumulate and form bigger clusters when the Ce loading increased to 7 wt%. GC-MS results showed that the hydrocarbons and esters in bio-oils increased with Ce loading, while those of ketones and aldehydes decreased. The possible catalytic reaction pathway was accordingly proposed. • Effect of Ni:Ce of Ni-xCe/CNTs were studied for the hydrothermal liquefaction of Tetra Pak. • Ce enhanced deoxygenation and decarbonylation reactions to form higher hydrocarbon. • Ni–5Ce/CNTs showed best catalytic activity, and the possible reaction pathways were analyzed." @default.
- W4293385909 created "2022-08-28" @default.
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- W4293385909 date "2022-12-01" @default.
- W4293385909 modified "2023-10-06" @default.
- W4293385909 title "Catalytic hydrothermal liquefaction of Tetra Pak with Ni-xCe/CNTs" @default.
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- W4293385909 doi "https://doi.org/10.1016/j.energy.2022.125302" @default.
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