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• W4293493479 endingPage "2206377" @default.
• W4293493479 startingPage "2206377" @default.
• W4293493479 abstract "MXenes constitute a rapidly growing family of 2D materials that are promising for optoelectronic applications because of numerous attractive properties, including high electrical conductivity. However, the most widely used titanium carbide (Ti3C2Tx) MXene transparent conductive electrode exhibits insufficient environmental stability and work function (WF), which impede practical applications Ti3C2Tx electrodes in solution-processed optoelectronics. Herein, Ti3C2Tx MXene film with a compact structure and a perfluorosulfonic acid (PFSA) barrier layer is presented as a promising electrode for organic light-emitting diodes (OLEDs). The electrode shows excellent environmental stability, high WF of 5.84 eV, and low sheet resistance RS of 97.4 Ω sq−1. The compact Ti3C2Tx structure after thermal annealing resists intercalation of moisture and environmental contaminants. In addition, the PFSA surface modification passivates interflake defects and modulates the WF. Thus, changes in the WF and RS are negligible even after 22 days of exposure to ambient air. The Ti3C2Tx MXene is applied for large-area, 10 × 10 passive matrix flexible OLEDs on substrates measuring 6 × 6 cm. This work provides a simple but efficient strategy to overcome both the limited environmental stability and low WF of MXene electrodes for solution-processable optoelectronics." @default.
• W4293493479 created "2022-08-29" @default.
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• W4293493479 date "2022-09-14" @default.
• W4293493479 modified "2023-10-15" @default.
• W4293493479 title "Overcoming the Limitations of MXene Electrodes for Solution‐Processed Optoelectronic Devices" @default.
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• W4293493479 doi "https://doi.org/10.1002/adma.202206377" @default.
• W4293493479 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/36037306" @default.
• W4293493479 hasPublicationYear "2022" @default.
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