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• W4293498883 abstract "Abstract The effect of N 2 discharge products on cyclohexane degradation over a MnO 2 / γ -Al 2 O 3 catalyst has been evaluated by feeding N 2 discharge products to the catalyst using a specially designed dielectric barrier discharge reactor. At a reaction temperature of 100 °C, the cyclohexane conversion increased from 2.46% (without N 2 discharge products) to 26.3% (with N 2 discharge products). N- and O-containing by-product (3, 4-dehydroproline) was found on the catalyst surface using gas chromatograph-mass spectrometry identification, in which C=N–C and C=N–H bonds were also confirmed from x-ray photoelectron spectroscopy analysis results. Operando analysis results using diffuse reflectance infrared Fourier transform spectroscopy revealed that N atoms can react with surface H 2 O possibly to NH and OH reactive species that have reactivities to promote CO oxidation to CO 2 . The mechanism of N-atom-driven cyclohexane degradation to CO and CO 2 is proposed." @default.
• W4293498883 created "2022-08-29" @default.
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• W4293498883 date "2023-01-06" @default.
• W4293498883 modified "2023-09-27" @default.
• W4293498883 title "Investigation of cyclohexane catalytic degradation driven by N atoms from N₂ discharges" @default.
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• W4293498883 doi "https://doi.org/10.1088/2058-6272/ac8a40" @default.
• W4293498883 hasPublicationYear "2023" @default.
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