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- W4293559862 abstract "Herein, the lipase-catalyzed ring-opening copolymerization of the diethylene diselenide carbonate dimer (SeC) with its analogue macrocycle (1,3,12,14-Tetraoxacyclodocosane-2,13-dione, TDC) was explored, and the small-ring carbonate (TMC) was used as control. The structure and composition of the diselenide-functionalized long-chain polycarbonates were confirmed by NMR and FTIR. The 13C NMR and 77Se NMR showed that the copolymers observed random sequence. Moreover, the kinetic process of TDC + SeC copolymerization demonstrated a faster polymerization rate and higher conversion of SeC in comparison with TMC + SeC. Besides, the copolymers exhibited ROS-responsive behaviors when exposed to the oxidizing environment owing to the diselenide groups, which was confirmed by UV–vis, DLS and TEM. Therefore, the ROS responsiveness facilitated potential application for the diselenide-functionalized copolymers." @default.
- W4293559862 created "2022-08-30" @default.
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- W4293559862 date "2022-10-01" @default.
- W4293559862 modified "2023-10-15" @default.
- W4293559862 title "Lipase-catalyzed ring-opening copolymerization of macrocycles for diselenide-functionalized long-chain polycarbonate: Synthesis, kinetic process and ROS responsiveness" @default.
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- W4293559862 doi "https://doi.org/10.1016/j.reactfunctpolym.2022.105385" @default.
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