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- W4293574906 abstract "We report that the atomic-scale vibrational coupling at the solid-fluid interface can substantially alter the interfacial properties such as wettability and fluid slip. The wettability of water droplets on substrates subjected to various vibrational frequencies is studied using molecular dynamics simulation. The contact angle increases (i.e., becomes more hydrophobic) when the oscillation frequency of the substrate matches the intermolecular bending frequency of liquid water. We investigate the underlying mechanism by examining the dynamics of water molecules at the interface and find that the temporal contact between the solid and fluid is shorter when the frequencies match, resulting in weak solid-fluid adsorption. We further report that the vibrational match at the interface reduces wall-fluid friction and enhances water transport through the nanopore. Our findings demonstrate the importance of the atomic-scale vibrational coupling at the solid-fluid interface on the physicochemical behavior of nanodevices and biological nanochannels." @default.
- W4293574906 created "2022-08-30" @default.
- W4293574906 creator A5068723726 @default.
- W4293574906 creator A5073593948 @default.
- W4293574906 date "2022-08-30" @default.
- W4293574906 modified "2023-10-17" @default.
- W4293574906 title "Effect of interfacial vibrational coupling on surface wettability and water transport" @default.
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- W4293574906 doi "https://doi.org/10.1103/physreve.106.025106" @default.
- W4293574906 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/36109939" @default.
- W4293574906 hasPublicationYear "2022" @default.
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